Controlled Growth and Disorder Mitigation of GaAs1– x Sb x /InAs Core–Shell Quantum Wires
Abstract We report the growth and transport properties of GaAs1–xSbx/InAs core–shell nanowires. Compared with the well-studied GaAs-InAs system, incorporating Sb substantially reduces the lattice mismatch between the core and shell. Accordingly, both the nanowire crystal quality and device performance improved significantly. Increasing x from 0.15 to 0.35, the density of crystalline defects, such as stacking faults in the InAs shell, decreases by half. Moreover, the field-effect mobility increases from 3850 cm2/(V s) to 4800 cm2/(V s), consistent with the reduction of the lattice mismatch. The incorporation of Sb makes the nanowire easier to pinch off via the gate voltage, enhancing the electric field tunability over the nanowire. Magneto-conductance measurements reveal Aharonov-Bohm-like oscillations, suggesting a phase-coherent tubular InAs shell. Our results identify lattice mismatch as a critical disorder source in core–shell nanowires and provide a practical route toward low-disorder core–shell quantum devices.
Authors
- Dong Pan (ORCID: https://orcid.org/0000-0003-2067-6983)
- Ran Zhuo (ORCID: https://orcid.org/0000-0003-1228-4496)
- Runan Shang
- Yanlin Wu (ORCID: https://orcid.org/0000-0002-1372-1822)
- Haitao Zhang (ORCID: https://orcid.org/0000-0002-1639-4089)
- Donghai Li (ORCID: https://orcid.org/0000-0003-1862-8333)
- Wenlong Yang
- Haiyan Shi
- 侯曦宇
- Sijun Chen
- Huading Song
- Zhichuan Wang
- Jinjin Bai
Institutions
- Chinese Academy of Sciences (CN)
- Southern University of Science and Technology (CN)
- Beijing Academy of Quantum Information Sciences (CN)
- University of Chinese Academy of Sciences (CN)
- Quantum Science Center of Guangdong-Hong Kong-Macao Greater Bay Area (CN)
Publication Details
- Journal
- The Journal of Physical Chemistry Letters
- Published
- 2026-11-06
- DOI
- https://doi.org/10.1021/acs.jpclett.6c02953
- Primary Topic
- Nanowire Synthesis and Applications
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- National Natural Science Foundation of China
- Chinese Academy of Sciences
- Youth Innovation Promotion Association of the Chinese Academy of Sciences
- National Science and Technology Major Project
- Beijing Municipal Natural Science Foundation
- National Key Research and Development Program of China