Controlled Growth and Disorder Mitigation of GaAs1– x Sb x /InAs Core–Shell Quantum Wires

Abstract We report the growth and transport properties of GaAs1–xSbx/InAs core–shell nanowires. Compared with the well-studied GaAs-InAs system, incorporating Sb substantially reduces the lattice mismatch between the core and shell. Accordingly, both the nanowire crystal quality and device performance improved significantly. Increasing x from 0.15 to 0.35, the density of crystalline defects, such as stacking faults in the InAs shell, decreases by half. Moreover, the field-effect mobility increases from 3850 cm2/(V s) to 4800 cm2/(V s), consistent with the reduction of the lattice mismatch. The incorporation of Sb makes the nanowire easier to pinch off via the gate voltage, enhancing the electric field tunability over the nanowire. Magneto-conductance measurements reveal Aharonov-Bohm-like oscillations, suggesting a phase-coherent tubular InAs shell. Our results identify lattice mismatch as a critical disorder source in core–shell nanowires and provide a practical route toward low-disorder core–shell quantum devices.

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Publication Details

Journal
The Journal of Physical Chemistry Letters
Published
2026-11-06
DOI
https://doi.org/10.1021/acs.jpclett.6c02953
Primary Topic
Nanowire Synthesis and Applications
Type
article
Field-Weighted Citation Impact
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Controlled Growth and Disorder Mitigation of GaAs1– x Sb x /InAs Core–Shell Quantum Wires

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1 links
The Journal of Physical Chemistry Letters
Nanowire Synthesis and Applications
article

Controlled Growth and Disorder Mitigation of GaAs1– x Sb x /InAs Core–Shell Quantum Wires

Dong Pan, Ran Zhuo, Runan Shang, Yanlin Wu, Haitao Zhang, Donghai Li, Wenlong Yang, Haiyan Shi, 侯曦宇, Sijun Chen, Huading Song, Zhichuan Wang, Jinjin Bai
article en

Abstract

Abstract We report the growth and transport properties of GaAs1–xSbx/InAs core–shell nanowires. Compared with the well-studied GaAs-InAs system, incorporating Sb substantially reduces the lattice mismatch between the core and shell. Accordingly, both the nanowire crystal quality and device performance improved significantly. Increasing x from 0.15 to 0.35, the density of crystalline defects, such as stacking faults in the InAs shell, decreases by half. Moreover, the field-effect mobility increases from 3850 cm2/(V s) to 4800 cm2/(V s), consistent with the reduction of the lattice mismatch. The incorporation of Sb makes the nanowire easier to pinch off via the gate voltage, enhancing the electric field tunability over the nanowire. Magneto-conductance measurements reveal Aharonov-Bohm-like oscillations, suggesting a phase-coherent tubular InAs shell. Our results identify lattice mismatch as a critical disorder source in core–shell nanowires and provide a practical route toward low-disorder core–shell quantum devices.

The Journal of Physical Chemistry Letters
Chinese Academy of Sciences (CN), Southern University of Science and Technology (CN), Beijing Academy of Quantum Information Sciences (CN), University of Chinese Academy of Sciences (CN), Quantum Science Center of Guangdong-Hong Kong-Macao Greater Bay Area (CN)
National Natural Science Foundation of China, Chinese Academy of Sciences, Youth Innovation Promotion Association of the Chinese Academy of Sciences, National Science and Technology Major Project, Beijing Municipal Natural Science Foundation, National Key Research and Development Program of China
Openalex Percentile: Top 35%
Nanowire Synthesis and Applications
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