Direct‐Write 3D Printing of TIM ‐Free Heat Sinks for Enhanced Chip‐Level Thermal Management
ABSTRACT Compared with traditional thermal interface material (TIM) systems, the TIM‐free heat dissipation system proposed in the study removes the separate TIM layer by using a 3D‐printed monolithic structure, thereby reducing the number of thermal interfaces in the heat path. The integrated design allows for custom‐designed, lightweight, and compact structures directly printed onto heat sources, enhancing thermal management efficiency. In this study, we introduce a novel silicone‐based thermal conductive gel, named TIM‐free, achieving a thermal conductivity of up to 1.69 W m −1 K −1 , a total thermal resistance as low as 5.31 × 10 −4 m 2 K W −1 , a storage modulus as low as 392.8 Pa, and an elongation at break of up to 5.44%. Moreover, the TIM‐free gel exhibits excellent printability and can be directly written into 3D heat sink structures. In thermal management tests, the TIM‐free gel was printed directly onto ceramic heaters; compared with setups without any TIM, the temperature of the ceramic heater equipped with the printed TIM‐free heat sink was reduced by 10°C. This approach is particularly suitable for high‐power‐density, next‐generation electronics requiring efficient and space‐saving thermal solutions.
Authors
- Chang‐Ping Feng (ORCID: https://orcid.org/0000-0003-3070-9021)
- Shuai Zhou (ORCID: https://orcid.org/0000-0002-5906-2607)
- Lei Hou (ORCID: https://orcid.org/0000-0002-2874-9326)
- Fang Wei (ORCID: https://orcid.org/0009-0002-0270-4282)
- Yu‐Zhong Wang (ORCID: https://orcid.org/0000-0001-8694-4106)
- Hongbo Lan (ORCID: https://orcid.org/0000-0002-0959-5413)
- Jian Song
- Wen‐Tao Hu
- Chen‐Yu Zhang
- Jin‐Chao Ji
- Fei Wang
- Ji‐Jin Wu
- Zheng‐Ting Song (ORCID: https://orcid.org/0009-0007-7731-4437)
Institutions
- Sichuan University (CN)
- State Key Laboratory of Polymer Materials Engineering (CN)
- Qingdao University of Technology (CN)
Publication Details
- Journal
- Journal of Applied Polymer Science
- Published
- 2026-11-06
- DOI
- https://doi.org/10.1002/app.71756
- Primary Topic
- Thermal properties of materials
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Department of Education of Shandong Province
- National Natural Science Foundation of China
- China Postdoctoral Science Foundation
- Sichuan University
- Natural Science Foundation of Shandong Province