Thermodynamic Evidence for Multiple Field-Induced Phases in an Anisotropic Kagome Antiferromagnet

Kagome antiferromagnets are predicted to host exotic field-induced phases, yet experimental identification of their thermodynamic signatures remains challenging. Here we combine specific heat ($C$) and ultrasound measurements up to 36 T and down to 0.5 K to map the $H-T$ phase diagram of the anisotropic kagome magnet Y$_3$Cu$_9$(OH)$_{19}$Cl$_8$. We show that the suppression of long-range antiferromagnetic order with field at $\sim 15$ T approximately coincides with the onset of the unconventional $1/6$ (or $1/9$) magnetization plateau previously observed in this system. The attenuation (and sound velocity) then intriguingly increases down to 0.5 K just at $μ_0H = 15$ T, and $C/T$ becomes temperature independent. Moreover, our measurements are consistent with the opening of a spin gap $Δ_0\simeq3.5\pm 0.3$ K within the plateau and reveal a further compressible (ungapped) phase beyond the plateau phase, unveiling a rich sequence of field-induced phases in this quantum magnet.

Authors

Publication Details

Journal
arXiv (Cornell University)
Published
2026-11-03
DOI
https://doi.org/10.48550/arxiv.2611.04675
Primary Topic
Advanced Condensed Matter Physics
Type
preprint
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preprint

Thermodynamic Evidence for Multiple Field-Induced Phases in an Anisotropic Kagome Antiferromagnet

P. Puphal, A. De Muer, D. LeBoeuf, N. Wack et al.
arXiv (Cornell University)
Advanced Condensed Matter Physics
preprint

Thermodynamic Evidence for Multiple Field-Induced Phases in an Anisotropic Kagome Antiferromagnet

P. Puphal, A. De Muer, D. LeBoeuf, N. Wack, C. Marcenat, M. Schuchard, Q. Barthélemy, T. Klein
preprint en

Abstract

Kagome antiferromagnets are predicted to host exotic field-induced phases, yet experimental identification of their thermodynamic signatures remains challenging. Here we combine specific heat ($C$) and ultrasound measurements up to 36 T and down to 0.5 K to map the $H-T$ phase diagram of the anisotropic kagome magnet Y$_3$Cu$_9$(OH)$_{19}$Cl$_8$. We show that the suppression of long-range antiferromagnetic order with field at $\sim 15$ T approximately coincides with the onset of the unconventional $1/6$ (or $1/9$) magnetization plateau previously observed in this system. The attenuation (and sound velocity) then intriguingly increases down to 0.5 K just at $μ_0H = 15$ T, and $C/T$ becomes temperature independent. Moreover, our measurements are consistent with the opening of a spin gap $Δ_0\simeq3.5\pm 0.3$ K within the plateau and reveal a further compressible (ungapped) phase beyond the plateau phase, unveiling a rich sequence of field-induced phases in this quantum magnet.

arXiv (Cornell University)
Advanced Condensed Matter Physics
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