Long-Term Environmental Durability of Recycled Textile-Low-Density Polyethylene Composites Reinforced with Plant Fibers: Mass Uptake, Flexural Stability, and Microbial Colonization

Recycled textile-polyethylene composites combine heterogeneous polymer and cellulosic phases whose long-term response to moisture and microbial colonization determines their suitability for building products. To the best of the authors’ knowledge, this is the first study to couple one-year, real-environment (non-accelerated) exposure of product-scale composites made from mixed post-consumer textile waste with mechanical testing and amplicon-based profiling of the viable surface microbiota, thereby linking material durability and biological colonization in a single dataset. In this study, recycled textile-low-density polyethylene (LDPE) composites produced by intrusion or extrusion and reinforced with 3 wt.% coconut or sisal fibers, together with an unreinforced reference and selected brushed-surface variants, were evaluated after 12 months in soil or water. Mass change and three-point flexural properties were quantified using five specimens per condition, and the culturable surface communities were characterized by 16S rRNA (V3–V4) and ITS1 amplicon sequencing. Mass gain remained low (0.116–0.580%), although water exposure and surface brushing significantly increased uptake. Across all material-exposure variants, flexural strain at break, flexural stress at break, flexural modulus, and maximum flexural stress decreased by only 0.3–1.1%, and every uncertainty-normalized shift remained below 0.5 propagated standard errors. Bacterial communities were dominated by Pseudomonas, Serratia, or Bacillus, whereas fungal profiles separated into Naganishia/Filobasidium-rich and Mucor-dominated assemblages. A literature-based trait analysis revealed high cumulative abundances of genera with documented cellulose- and ester-hydrolyzing capacity and, among bacteria, polyethylene/alkane-oxidizing capacity. The results indicate persistent biological colonization of the composite surfaces, whereas bulk flexural performance remained essentially unchanged after one year of environmental exposure.

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Publication Details

Journal
Materials
Published
2026-10-26
DOI
https://doi.org/10.3390/ma19214504
Primary Topic
Natural Fiber Reinforced Composites
Type
article
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article

Long-Term Environmental Durability of Recycled Textile-Low-Density Polyethylene Composites Reinforced with Plant Fibers: Mass Uptake, Flexural Stability, and Microbial Colonization

Wiesław Kaca, Marcin Małek, Norbert Lipka
Materials
Natural Fiber Reinforced Composites
article

Long-Term Environmental Durability of Recycled Textile-Low-Density Polyethylene Composites Reinforced with Plant Fibers: Mass Uptake, Flexural Stability, and Microbial Colonization

Wiesław Kaca, Marcin Małek, Norbert Lipka
article en

Abstract

Recycled textile-polyethylene composites combine heterogeneous polymer and cellulosic phases whose long-term response to moisture and microbial colonization determines their suitability for building products. To the best of the authors’ knowledge, this is the first study to couple one-year, real-environment (non-accelerated) exposure of product-scale composites made from mixed post-consumer textile waste with mechanical testing and amplicon-based profiling of the viable surface microbiota, thereby linking material durability and biological colonization in a single dataset. In this study, recycled textile-low-density polyethylene (LDPE) composites produced by intrusion or extrusion and reinforced with 3 wt.% coconut or sisal fibers, together with an unreinforced reference and selected brushed-surface variants, were evaluated after 12 months in soil or water. Mass change and three-point flexural properties were quantified using five specimens per condition, and the culturable surface communities were characterized by 16S rRNA (V3–V4) and ITS1 amplicon sequencing. Mass gain remained low (0.116–0.580%), although water exposure and surface brushing significantly increased uptake. Across all material-exposure variants, flexural strain at break, flexural stress at break, flexural modulus, and maximum flexural stress decreased by only 0.3–1.1%, and every uncertainty-normalized shift remained below 0.5 propagated standard errors. Bacterial communities were dominated by Pseudomonas, Serratia, or Bacillus, whereas fungal profiles separated into Naganishia/Filobasidium-rich and Mucor-dominated assemblages. A literature-based trait analysis revealed high cumulative abundances of genera with documented cellulose- and ester-hydrolyzing capacity and, among bacteria, polyethylene/alkane-oxidizing capacity. The results indicate persistent biological colonization of the composite surfaces, whereas bulk flexural performance remained essentially unchanged after one year of environmental exposure.

MaterialsVol. 19(21)
Jan Kochanowski University (PL), Military University of Technology in Warsaw (PL)
Openalex Percentile: Top 26%
Natural Fiber Reinforced Composites
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