Assessing the Impact of Incorporating Bias-Adjusted Satellite Observations into Global Data Fusion for Ground-level Health-Related Ozone Metrics

Understanding global ground-level ozone is hindered by significant monitoring gaps. To address this, we introduce a Bayesian Maximum Entropy data fusion framework that includes satellite ozone observations, generating a global 0.1° surface ozone dataset (2005–2022). Satellite observations (IASI+GOME2, OMI/MLS), adjusted to ground-level estimates, were analyzed using Flexible Regionalized Air Quality Model Performance to correct biases and estimate variance. Ground observations (hard data) and satellite-derived estimates (soft data) were then integrated, using a composite of 10 atmospheric chemistry models and 3 reanalyses as the global spatial-temporal trend. Cross-validations demonstrated high overall accuracy (R 2 = 0.83; RMSE = 3.73 ppb). Although integrating satellite-derived soft data yields only marginal performance gains in densely monitored areas, it substantially reduces model uncertainties and improves model accuracy across large spatial gaps. Notably, for the furthest unmonitored gap group at a 20° checkerboard, including satellite data increased R 2 by 25.9% and decreased RMSE by 21.1% after the integration. Applying this optimized data fusion configuration from 2005 to 2022, global population-weighted ozone is estimated to have increased by 0.21 ppb/decade. Consequently, the global population exposed to ozone levels exceeding 50 ppb more than doubled over this 18-year period, rising from 17.2% to 41.0%.

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Publication Details

Journal
ChemRxiv
Published
2026-10-26
DOI
https://doi.org/10.26434/chemrxiv.15011001/v2
Primary Topic
Air Quality Monitoring and Forecasting
Type
preprint

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preprint

Assessing the Impact of Incorporating Bias-Adjusted Satellite Observations into Global Data Fusion for Ground-level Health-Related Ozone Metrics

Rebecca R. Buchholz, Kai-Lan Chang, J. Jason West, Owen R. Cooper et al.
ChemRxiv
Air Quality Monitoring and Forecasting
preprint

Assessing the Impact of Incorporating Bias-Adjusted Satellite Observations into Global Data Fusion for Ground-level Health-Related Ozone Metrics

Rebecca R. Buchholz, Kai-Lan Chang, J. Jason West, Owen R. Cooper, Juan Cuesta, Marc L. Serre, Makoto Deushi, J. R. Ziemke, Luke D. Oman, Zhen Qu, Hantao Wang, Praful Dodda, Meiyun Lin, Kazuyuki Miyazaki, George E. Heidkamp
preprint en

Abstract

Understanding global ground-level ozone is hindered by significant monitoring gaps. To address this, we introduce a Bayesian Maximum Entropy data fusion framework that includes satellite ozone observations, generating a global 0.1° surface ozone dataset (2005–2022). Satellite observations (IASI+GOME2, OMI/MLS), adjusted to ground-level estimates, were analyzed using Flexible Regionalized Air Quality Model Performance to correct biases and estimate variance. Ground observations (hard data) and satellite-derived estimates (soft data) were then integrated, using a composite of 10 atmospheric chemistry models and 3 reanalyses as the global spatial-temporal trend. Cross-validations demonstrated high overall accuracy (R 2 = 0.83; RMSE = 3.73 ppb). Although integrating satellite-derived soft data yields only marginal performance gains in densely monitored areas, it substantially reduces model uncertainties and improves model accuracy across large spatial gaps. Notably, for the furthest unmonitored gap group at a 20° checkerboard, including satellite data increased R 2 by 25.9% and decreased RMSE by 21.1% after the integration. Applying this optimized data fusion configuration from 2005 to 2022, global population-weighted ozone is estimated to have increased by 0.21 ppb/decade. Consequently, the global population exposed to ozone levels exceeding 50 ppb more than doubled over this 18-year period, rising from 17.2% to 41.0%.

ChemRxiv
NSF National Center for Atmospheric Research (US), California Institute of Technology (US), Centre National de la Recherche Scientifique (FR), Goddard Space Flight Center (US), Jet Propulsion Laboratory (US), North Carolina State University (US), Cooperative Institute for Research in Environmental Sciences (US), NOAA Geophysical Fluid Dynamics Laboratory (US), Université Paris-Est Créteil (FR), Université Paris Cité (FR), NOAA Chemical Sciences Laboratory (US), Laboratoire Interuniversitaire des Systèmes Atmosphériques (FR), Meteorological Research Institute (JP)
National Aeronautics and Space Administration, National Oceanic and Atmospheric Administration
Air Quality Monitoring and Forecasting
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