Comparative study of second harmonic generation at 1030 nm in BiBO and LBO crystals using a 57 W picosecond laser

We present a systematic experimental comparison of second-harmonic generation (SHG) in bismuth triborate (BiBO) and lithium triborate (LBO) nonlinear crystals, driven by a 1.3 ps, 91 kHz laser at 1030 nm with up to 57 W of average input power. Both crystals yielded 32 W of second harmonic (SH) output at 515 nm, corresponding to a conversion efficiency of 56%, which to the best of our knowledge represents the highest SH output power reported in the green spectral region using a BiBO crystal. Power dependence, long-term stability, beam quality, pulse duration, spectral properties, thermal effects, and angular acceptance bandwidth are characterized and directly compared for both crystals. These results provide quantitative performance benchmarks to guide the selection of nonlinear crystals for high-average-power, ultrashort-pulse frequency conversion near 1030 nm.