Purely Equatorial Lasing in Spherical Liquid Crystal Polymer Microlasers with Bipolar Refractive Index Profile

ABSTRACT Liquid crystal whispering gallery mode (WGM) microlasers show high sensitivity to external stimuli and distinct spectral features, rendering them ideally suited for various sensing applications. They also offer intrinsic anisotropic optical properties, which can be used to shape and manipulate light even inside spatially highly symmetric structures. Here, we report the fabrication of a spherical bipolar liquid crystal polymer microlaser that tightly confines the optical path of WGMs to the equatorial plane. By controlled anchoring of the liquid crystal mesogens followed by polymerization, a fixed refractive index profile is formed within the spherical microcavity. Consequently, only transverse electric (TE) modes oscillating in the equatorial plane experience the high extraordinary refractive index, allowing to confine lasing into a single plane. Furthermore, we observe a characteristic splitting into sub‐modes. By combining hyperspectral imaging, optical modeling, and theoretical calculations, we show that the observed sub‐modes originate from the lifting of the energy degeneracy of azimuthal WGMs. The unique ability to confine lasing into a single plane makes these spherical microlasers independent of the exact position of the pump beam, which allows consistent localized sensing, especially in combination with fast point scanning microscopes or inside highly dynamic biological environments.