Distribution of TENORM-contaminated soils in residential areas of Bangka Island, Indonesia

Radioactive contamination in residential areas of Bangka Island, Indonesia, a major tin- and rare earth-producing region, has rarely been studied, although material stored near mineral-processing workshops may pose a long-term health risk. We collected 46 soil samples around 9 mineral-processing workshops in the Selindung District, Pangkal Pinang City: residential soils from 20 locations at two depths ( n = 40) and 6 workshop-related sediments. High-purity germanium detector analysis showed that 13 of the 40 residential soil samples exceeded the screening criteria of the IAEA Safety Standards Series No. RS-G-1.7 for naturally occurring radioactive material. Residential contamination was highly heterogeneous and was not explained by a simple monotonic distance relationship (Spearman’s ρ = −0.12, p = 0.61). Two upper outliers occurred at 5 and 10 m from the nearest workshops, including the maximum residential activity of 12,992 Bq/kg detected at 5 m, in areas frequently accessed by local residents. Five of 17 locations with quantifiable paired measurements (including 1 tied pair; n = 16 for the Wilcoxon signed-rank test) showed higher activity at 20 cm than at 10 cm, and the paired depth difference was not statistically significant (Wilcoxon p = 0.079), indicating an irregular rather than consistently surface-dominated vertical distribution. Screening-level outdoor annual effective doses for the quantifiable residential samples ranged from 0.051 to 8.46 mSv/y (median 0.42 mSv/y), with the maximum obtained 5 m from a workshop. Nuclide composition analysis further revealed that the activity concentrations of the 238 U and 232 Th series increased with total radioactivity, whereas 40 K showed only a weak correlation. Maximum activities of 238 U and 232 Th approached levels reported by the IAEA for high-purity monazite sand (6,000–20,000 Bq/kg). These findings demonstrate spatial and vertical heterogeneity of technologically enhanced naturally occurring radioactive material in residential zones, indicating a need for site-specific assessment and long-term monitoring.

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PLoS ONE
Published
2026-10-05
DOI
https://doi.org/10.1371/journal.pone.0348187
Primary Topic
Radioactivity and Radon Measurements
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article
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article

Distribution of TENORM-contaminated soils in residential areas of Bangka Island, Indonesia

Cici Wulandari, Kan Shimazaki, Yo Ishigaki, Sidik Permana et al.
PLoS ONE
Radioactivity and Radon Measurements
article

Distribution of TENORM-contaminated soils in residential areas of Bangka Island, Indonesia

Cici Wulandari, Kan Shimazaki, Yo Ishigaki, Sidik Permana, Harrizki Arie Pradana, Katsumi Shozugawa, Adi Rahmansyah, Kazunori Hayashi, Ryo Ichimiya
article en

Abstract

Radioactive contamination in residential areas of Bangka Island, Indonesia, a major tin- and rare earth-producing region, has rarely been studied, although material stored near mineral-processing workshops may pose a long-term health risk. We collected 46 soil samples around 9 mineral-processing workshops in the Selindung District, Pangkal Pinang City: residential soils from 20 locations at two depths ( n = 40) and 6 workshop-related sediments. High-purity germanium detector analysis showed that 13 of the 40 residential soil samples exceeded the screening criteria of the IAEA Safety Standards Series No. RS-G-1.7 for naturally occurring radioactive material. Residential contamination was highly heterogeneous and was not explained by a simple monotonic distance relationship (Spearman’s ρ = −0.12, p = 0.61). Two upper outliers occurred at 5 and 10 m from the nearest workshops, including the maximum residential activity of 12,992 Bq/kg detected at 5 m, in areas frequently accessed by local residents. Five of 17 locations with quantifiable paired measurements (including 1 tied pair; n = 16 for the Wilcoxon signed-rank test) showed higher activity at 20 cm than at 10 cm, and the paired depth difference was not statistically significant (Wilcoxon p = 0.079), indicating an irregular rather than consistently surface-dominated vertical distribution. Screening-level outdoor annual effective doses for the quantifiable residential samples ranged from 0.051 to 8.46 mSv/y (median 0.42 mSv/y), with the maximum obtained 5 m from a workshop. Nuclide composition analysis further revealed that the activity concentrations of the 238 U and 232 Th series increased with total radioactivity, whereas 40 K showed only a weak correlation. Maximum activities of 238 U and 232 Th approached levels reported by the IAEA for high-purity monazite sand (6,000–20,000 Bq/kg). These findings demonstrate spatial and vertical heterogeneity of technologically enhanced naturally occurring radioactive material in residential zones, indicating a need for site-specific assessment and long-term monitoring.

PLoS ONEVol. 21(10)
Bandung Institute of Technology (ID), The University of Tokyo (JP), Kindai University (JP)
Openalex Percentile: Top 8%
Radioactivity and Radon Measurements
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