Distribution of TENORM-contaminated soils in residential areas of Bangka Island, Indonesia
Radioactive contamination in residential areas of Bangka Island, Indonesia, a major tin- and rare earth-producing region, has rarely been studied, although material stored near mineral-processing workshops may pose a long-term health risk. We collected 46 soil samples around 9 mineral-processing workshops in the Selindung District, Pangkal Pinang City: residential soils from 20 locations at two depths ( n = 40) and 6 workshop-related sediments. High-purity germanium detector analysis showed that 13 of the 40 residential soil samples exceeded the screening criteria of the IAEA Safety Standards Series No. RS-G-1.7 for naturally occurring radioactive material. Residential contamination was highly heterogeneous and was not explained by a simple monotonic distance relationship (Spearman’s ρ = −0.12, p = 0.61). Two upper outliers occurred at 5 and 10 m from the nearest workshops, including the maximum residential activity of 12,992 Bq/kg detected at 5 m, in areas frequently accessed by local residents. Five of 17 locations with quantifiable paired measurements (including 1 tied pair; n = 16 for the Wilcoxon signed-rank test) showed higher activity at 20 cm than at 10 cm, and the paired depth difference was not statistically significant (Wilcoxon p = 0.079), indicating an irregular rather than consistently surface-dominated vertical distribution. Screening-level outdoor annual effective doses for the quantifiable residential samples ranged from 0.051 to 8.46 mSv/y (median 0.42 mSv/y), with the maximum obtained 5 m from a workshop. Nuclide composition analysis further revealed that the activity concentrations of the 238 U and 232 Th series increased with total radioactivity, whereas 40 K showed only a weak correlation. Maximum activities of 238 U and 232 Th approached levels reported by the IAEA for high-purity monazite sand (6,000–20,000 Bq/kg). These findings demonstrate spatial and vertical heterogeneity of technologically enhanced naturally occurring radioactive material in residential zones, indicating a need for site-specific assessment and long-term monitoring.
Authors
- Cici Wulandari (ORCID: https://orcid.org/0000-0001-9903-9850)
- Kan Shimazaki (ORCID: https://orcid.org/0000-0002-7726-7390)
- Yo Ishigaki (ORCID: https://orcid.org/0000-0001-7284-0381)
- Sidik Permana (ORCID: https://orcid.org/0000-0002-0667-3041)
- Harrizki Arie Pradana (ORCID: https://orcid.org/0000-0002-8814-0467)
- Katsumi Shozugawa (ORCID: https://orcid.org/0000-0001-6945-2927)
- Adi Rahmansyah (ORCID: https://orcid.org/0000-0002-5267-9049)
- Kazunori Hayashi (ORCID: https://orcid.org/0009-0002-2977-8353)
- Ryo Ichimiya
Institutions
- Bandung Institute of Technology (ID)
- The University of Tokyo (JP)
- Kindai University (JP)
Publication Details
- Journal
- PLoS ONE
- Published
- 2026-10-05
- DOI
- https://doi.org/10.1371/journal.pone.0348187
- Primary Topic
- Radioactivity and Radon Measurements
- Type
- article
- Field-Weighted Citation Impact
- 0.00