Room‐Temperature Anomalous Hall Effect and Out‐of‐Plane Spin–Orbit Torques in CoFe 2 O 4 ‐Buffered RuO 2

ABSTRACT Realizing room‐temperature out‐of‐plane spin currents remains a key challenge for low‐power perpendicular spin–orbit torque devices. Oxides with strong spin–orbit coupling are highly desirable spin sources for spintronic applications, and RuO 2 has recently attracted widespread attention owing to its excellent spin transport properties. However, the generation of out‐of‐plane spin polarization is limited to specific crystallographic orientations, restricting materials design flexibility and practical device integration. Here, we demonstrate that interfacial magnetic coupling between RuO 2 and an insulating ferromagnet can provide an effective route to circumvent this constraint. In RuO 2 (110)/CoFe 2 O 4 heterostructures, the interfacial coupling induces a net magnetization component in RuO 2 tilted toward the film plane, giving rise to a robust anomalous Hall effect up to room temperature. Spin‐torque ferromagnetic resonance measurements reveal a high spin–orbit torque efficiency of ∼0.18 in CoFe 2 O 4 ‐buffered RuO 2 , representing a sixfold enhancement compared with bare RuO 2 (110) films. Notably, the spin tilting of RuO 2 generates a distinct z‐polarized spin‐current component with a torque efficiency of ∼0.014, indicating that interfacial magnetic engineering enables out‐of‐plane spin polarization in RuO 2 (110). These results suggest interfacial magnetic modulation as a versatile strategy for realizing room‐temperature anomalous Hall effects and efficient spin–orbit torques in strongly spin–orbit coupled oxide heterostructures, opening new opportunities for oxide‐based spintronic applications.

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Publication Details

Journal
Advanced Functional Materials
Published
2026-09-29
DOI
https://doi.org/10.1002/adfm.78734
Primary Topic
Magnetic properties of thin films
Type
article
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Room‐Temperature Anomalous Hall Effect and Out‐of‐Plane Spin–Orbit Torques in CoFe 2 O 4 ‐Buffered RuO 2

Jine Zhang, Jirong Sun, Fengxia Hu, Guibin Lan et al.
Advanced Functional Materials
Magnetic properties of thin films
article

Room‐Temperature Anomalous Hall Effect and Out‐of‐Plane Spin–Orbit Torques in CoFe 2 O 4 ‐Buffered RuO 2

Jine Zhang, Jirong Sun, Fengxia Hu, Guibin Lan, Jie Zheng, Baogen Shen, Hao Wu, Yuansha Chen, Yunzhong Chen, Furong Han, Tao Zhu, Guoqiang Yu, 王登京, Daming Tian, Pengju Wang, Hongrui Zhang, Meng Yang Zhao, He Bai, Ziqi Han, Jirong Sun, Jianwang Cai, Cheng Zhang, Jing Zhang, Haodong Liu
article en

Abstract

ABSTRACT Realizing room‐temperature out‐of‐plane spin currents remains a key challenge for low‐power perpendicular spin–orbit torque devices. Oxides with strong spin–orbit coupling are highly desirable spin sources for spintronic applications, and RuO 2 has recently attracted widespread attention owing to its excellent spin transport properties. However, the generation of out‐of‐plane spin polarization is limited to specific crystallographic orientations, restricting materials design flexibility and practical device integration. Here, we demonstrate that interfacial magnetic coupling between RuO 2 and an insulating ferromagnet can provide an effective route to circumvent this constraint. In RuO 2 (110)/CoFe 2 O 4 heterostructures, the interfacial coupling induces a net magnetization component in RuO 2 tilted toward the film plane, giving rise to a robust anomalous Hall effect up to room temperature. Spin‐torque ferromagnetic resonance measurements reveal a high spin–orbit torque efficiency of ∼0.18 in CoFe 2 O 4 ‐buffered RuO 2 , representing a sixfold enhancement compared with bare RuO 2 (110) films. Notably, the spin tilting of RuO 2 generates a distinct z‐polarized spin‐current component with a torque efficiency of ∼0.014, indicating that interfacial magnetic engineering enables out‐of‐plane spin polarization in RuO 2 (110). These results suggest interfacial magnetic modulation as a versatile strategy for realizing room‐temperature anomalous Hall effects and efficient spin–orbit torques in strongly spin–orbit coupled oxide heterostructures, opening new opportunities for oxide‐based spintronic applications.

Advanced Functional Materials
Chinese Academy of Sciences (CN), China Spallation Neutron Source (CN), Songshan Lake Materials Laboratory (CN), Institute of Physics (CN), University of Chinese Academy of Sciences (CN), Ningbo Institute of Industrial Technology (CN), Wuhan University of Science and Technology (CN), Beihang University (CN)
Openalex Percentile: Top 14%
Magnetic properties of thin films
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