Weaker π-conjugation but longer 3MLCT lifetimes: a comparative ultrafast spectroscopic study of dinuclear pentacyanoferrate(II) complexes.

Two dinuclear pentacyanoferrate(II) complexes with different bridging ligands were prepared to investigate the effect of ligand conjugation on the photophysics of Fe(II) photosensitizers. Femtosecond transient absorption studies suggest that the MLCT lifetime and excited-state dynamics depend on both ligand conjugation and ligand flexibility in solution.

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Journal
PubMed
Published
2026-09-15
DOI
https://doi.org/10.1039/d6cp02581a
Primary Topic
Photochemistry and Electron Transfer Studies
Type
article
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article

Weaker π-conjugation but longer 3MLCT lifetimes: a comparative ultrafast spectroscopic study of dinuclear pentacyanoferrate(II) complexes.

Ferdi Karadaş, Kaixing Wang, Emir Utku Şekercileroğlu, Benjamin Dietzek-Ivanšić
PubMed
Photochemistry and Electron Transfer Studies
article

Weaker π-conjugation but longer 3MLCT lifetimes: a comparative ultrafast spectroscopic study of dinuclear pentacyanoferrate(II) complexes.

Ferdi Karadaş, Kaixing Wang, Emir Utku Şekercileroğlu, Benjamin Dietzek-Ivanšić
article en

Abstract

Two dinuclear pentacyanoferrate(II) complexes with different bridging ligands were prepared to investigate the effect of ligand conjugation on the photophysics of Fe(II) photosensitizers. Femtosecond transient absorption studies suggest that the MLCT lifetime and excited-state dynamics depend on both ligand conjugation and ligand flexibility in solution.

PubMed
Bilkent University (TR), Leibniz Institute of Photonic Technology (DE), Leibniz Institute of Surface Engineering (DE), Friedrich Schiller University Jena (DE), Leipzig University (DE)
Openalex Percentile: Top 12%
Photochemistry and Electron Transfer Studies
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