NaYF 4 : Er 3+ Nanoparticles‐Graphene Photodetector for High‐Responsivity 1.5 µm Narrowband Imaging and Multi‐Wavelength Sensing

ABSTRACT Silicon‐based photodetection in the 1.5 µm spectral window is important for next‐generation photonic systems, enabling critical applications in optical communication, LiDAR, and atmospheric gas sensing. Although erbium‐based upconversion photodetectors (UPDs) offer advantages in cost‐effective fabrication and stable spectral selectivity, their deployment is fundamentally limited by compromised responsivity, slow response times, and complex multilayer architectures that hinder scalability. Here, we report a UPD that synergistically integrates high‐efficiency Er‐based nanoparticles (ENPs) with an engineered graphene photogating architecture. Fabricated on SiO 2 /p+‐Si substrates, the optimized device achieves unparalleled performance metrics: a record‐high responsivity of 59.5 A/W at 1 V bias, millisecond‐scale response dynamics, and narrowband 1.5 µm detection. This exceptional performance originates from two synergistic mechanisms: the ENPs' high upconversion quantum yield (2.1%) and a substantial photoconductive gain (∼10 7 ) from the graphene photogating, increasing responsivity by a factor of 5 over conventional designs. Additionally, leveraging the intrinsic narrowband response of ENPs, we demonstrate a dual‐channel wavelength‐selective structure capable of effectively discriminating signals within the 1.5 µm band from those below 1.1 µm. This permits simultaneous multi‐wavelength detection, as demonstrated via spatially‐resolved imaging at 633 and 1523 nm. Combined with its fabrication simplicity and scalability, this work represents a significant leap forward for high‐performance UPDs.

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Publication Details

Journal
Advanced Functional Materials
Published
2026-09-15
DOI
https://doi.org/10.1002/adfm.78281
Primary Topic
Silicon Nanostructures and Photoluminescence
Type
article
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NaYF 4 : Er 3+ Nanoparticles‐Graphene Photodetector for High‐Responsivity 1.5 µm Narrowband Imaging and Multi‐Wavelength Sensing

Cun‐Zheng Ning, Ying Cui, Zhangyu Hou, Hao Sun et al.
Advanced Functional Materials
Silicon Nanostructures and Photoluminescence
article

NaYF 4 : Er 3+ Nanoparticles‐Graphene Photodetector for High‐Responsivity 1.5 µm Narrowband Imaging and Multi‐Wavelength Sensing

Cun‐Zheng Ning, Ying Cui, Zhangyu Hou, Hao Sun, Shipeng Yao, Jinhua Wu, Zhang Liang, Yongzhuo Li
article en

Abstract

ABSTRACT Silicon‐based photodetection in the 1.5 µm spectral window is important for next‐generation photonic systems, enabling critical applications in optical communication, LiDAR, and atmospheric gas sensing. Although erbium‐based upconversion photodetectors (UPDs) offer advantages in cost‐effective fabrication and stable spectral selectivity, their deployment is fundamentally limited by compromised responsivity, slow response times, and complex multilayer architectures that hinder scalability. Here, we report a UPD that synergistically integrates high‐efficiency Er‐based nanoparticles (ENPs) with an engineered graphene photogating architecture. Fabricated on SiO 2 /p+‐Si substrates, the optimized device achieves unparalleled performance metrics: a record‐high responsivity of 59.5 A/W at 1 V bias, millisecond‐scale response dynamics, and narrowband 1.5 µm detection. This exceptional performance originates from two synergistic mechanisms: the ENPs' high upconversion quantum yield (2.1%) and a substantial photoconductive gain (∼10 7 ) from the graphene photogating, increasing responsivity by a factor of 5 over conventional designs. Additionally, leveraging the intrinsic narrowband response of ENPs, we demonstrate a dual‐channel wavelength‐selective structure capable of effectively discriminating signals within the 1.5 µm band from those below 1.1 µm. This permits simultaneous multi‐wavelength detection, as demonstrated via spatially‐resolved imaging at 633 and 1523 nm. Combined with its fabrication simplicity and scalability, this work represents a significant leap forward for high‐performance UPDs.

Advanced Functional Materials
Shenzhen University (CN), Beijing Academy of Quantum Information Sciences (CN), Tsinghua University (CN)
Reduced inequalities
Openalex Percentile: Top 24%
Silicon Nanostructures and Photoluminescence
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