Mechanical Properties and Microstructure of Bonded Joints and Hybrid Structures with a 3D-Printed Honeycomb Core Modified with an Epoxy Matrix Filled with Recycled Polyurethane Foam

This article examines the reuse of waste polyurethane foam (PUF) as a material in line with circular economy principles. The main objective was to evaluate how crushed polyurethane filler of different bulk densities—35 kg·m−3 (PUF35), 60 kg·m−3 (PUF60), and their blends at 1–5 wt%—affects the mechanical behaviour and structural integrity of hybrid composite systems and bonded laminated joints. An epoxy resin matrix was combined with 3D-printed polylactide (PLA) honeycomb structures, with rectangular and hexagonal core geometries. Static tensile tests showed that the blended filler (PUF35/60) preserves tensile strength and increases the modulus of elasticity for both core geometries, reaching maximum values at 4 wt% (3.8 GPa for rectangular, 3.6 GPa for hexagonal cores). In bonded lap joints, 1 wt% PUF35 resulted in the highest tensile adhesive bond strength (13.3 MPa). SEM confirmed a high-quality phase interface and continuous adhesive contact between the epoxy matrix and the 3D-printed PLA surface, with dominant cohesive failure and effective mechanical anchoring of foam particles, even near local printing defects. The results confirm mechanically recycled PUF as a promising filler for advanced sandwich structures and adhesive systems.

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Publication Details

Journal
Materials
Published
2026-09-16
DOI
https://doi.org/10.3390/ma19183935
Primary Topic
Cellular and Composite Structures
Type
article
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article

Mechanical Properties and Microstructure of Bonded Joints and Hybrid Structures with a 3D-Printed Honeycomb Core Modified with an Epoxy Matrix Filled with Recycled Polyurethane Foam

Jaroslava Svobodová, Anna Rudawská, Petr Jirků, Miroslav Müller et al.
Materials
Cellular and Composite Structures
article

Mechanical Properties and Microstructure of Bonded Joints and Hybrid Structures with a 3D-Printed Honeycomb Core Modified with an Epoxy Matrix Filled with Recycled Polyurethane Foam

Jaroslava Svobodová, Anna Rudawská, Petr Jirků, Miroslav Müller, Rajesh Mishra, Petr Valášek, Jiří Marčan, Michal Penc
article en

Abstract

This article examines the reuse of waste polyurethane foam (PUF) as a material in line with circular economy principles. The main objective was to evaluate how crushed polyurethane filler of different bulk densities—35 kg·m−3 (PUF35), 60 kg·m−3 (PUF60), and their blends at 1–5 wt%—affects the mechanical behaviour and structural integrity of hybrid composite systems and bonded laminated joints. An epoxy resin matrix was combined with 3D-printed polylactide (PLA) honeycomb structures, with rectangular and hexagonal core geometries. Static tensile tests showed that the blended filler (PUF35/60) preserves tensile strength and increases the modulus of elasticity for both core geometries, reaching maximum values at 4 wt% (3.8 GPa for rectangular, 3.6 GPa for hexagonal cores). In bonded lap joints, 1 wt% PUF35 resulted in the highest tensile adhesive bond strength (13.3 MPa). SEM confirmed a high-quality phase interface and continuous adhesive contact between the epoxy matrix and the 3D-printed PLA surface, with dominant cohesive failure and effective mechanical anchoring of foam particles, even near local printing defects. The results confirm mechanically recycled PUF as a promising filler for advanced sandwich structures and adhesive systems.

MaterialsVol. 19(18)
Czech University of Life Sciences Prague (CZ), Jan Evangelista Purkyně University in Ústí nad Labem (CZ), Lublin University of Technology (PL)
Openalex Percentile: Top 20%
Cellular and Composite Structures
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