High Strain Rate Behavior and Energy Absorption of Nano-Silica Reinforced NR/NBR Blends: Temperature-Dependent SHPB Investigation

This study investigates the dynamic compressive behavior of natural rubber (NR)/acrylonitrile butadiene rubber (NBR) blends containing 20 phr carbon black and reinforced with 3 phr nano-silica under high strain-rate loading using a Split Hopkinson Pressure Bar (SHPB). The effects of temperature (−50 °C, 25 °C, and 100 °C) and blend composition on viscoelastic properties, densification, and energy absorption were evaluated. Dynamic mechanical analysis (DMA) showed that nano-silica increased the storage modulus (E′) and reduced the tan δ peak, indicating enhanced stiffness and stronger filler–matrix interactions. SHPB tests revealed a pronounced temperature dependence, with elastoplastic behavior at −50 °C and softening at 100 °C due to increased molecular mobility. The stress–strain response exhibited three characteristic stages: linear elasticity, plateau, and densification, with the highest densification strain observed at room temperature. Nano-silica significantly improved energy absorption at 10% and 30% strain, whereas unfilled blends showed greater damping with increasing NBR content at low temperatures. These findings demonstrate the combined influence of nano-silica, temperature, and blend composition on the impact resistance of NR/NBR composites.

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Publication Details

Journal
Journal of Macromolecular Science Part B
Published
2026-09-12
DOI
https://doi.org/10.1080/00222348.2026.2730377
Primary Topic
Polymer Nanocomposites and Properties
Type
article
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article

High Strain Rate Behavior and Energy Absorption of Nano-Silica Reinforced NR/NBR Blends: Temperature-Dependent SHPB Investigation

Hichem Tahraoui, Abdeltif Amrane, A. Chelli, Reguia Boudraa et al.
Journal of Macromolecular Science Part B
Polymer Nanocomposites and Properties
article

High Strain Rate Behavior and Energy Absorption of Nano-Silica Reinforced NR/NBR Blends: Temperature-Dependent SHPB Investigation

Hichem Tahraoui, Abdeltif Amrane, A. Chelli, Reguia Boudraa, Djalel Eddine Tria, Walid Elfalleh
article en

Abstract

This study investigates the dynamic compressive behavior of natural rubber (NR)/acrylonitrile butadiene rubber (NBR) blends containing 20 phr carbon black and reinforced with 3 phr nano-silica under high strain-rate loading using a Split Hopkinson Pressure Bar (SHPB). The effects of temperature (−50 °C, 25 °C, and 100 °C) and blend composition on viscoelastic properties, densification, and energy absorption were evaluated. Dynamic mechanical analysis (DMA) showed that nano-silica increased the storage modulus (E′) and reduced the tan δ peak, indicating enhanced stiffness and stronger filler–matrix interactions. SHPB tests revealed a pronounced temperature dependence, with elastoplastic behavior at −50 °C and softening at 100 °C due to increased molecular mobility. The stress–strain response exhibited three characteristic stages: linear elasticity, plateau, and densification, with the highest densification strain observed at room temperature. Nano-silica significantly improved energy absorption at 10% and 30% strain, whereas unfilled blends showed greater damping with increasing NBR content at low temperatures. These findings demonstrate the combined influence of nano-silica, temperature, and blend composition on the impact resistance of NR/NBR composites.

Journal of Macromolecular Science Part B
Centre National de la Recherche Scientifique (FR), Imam Mohammad ibn Saud Islamic University (SA), Polytechnic School of Algiers (DZ), Islamic University (BD), École Nationale Supérieure de Chimie de Rennes (FR), University Yahia Fares of Medea (DZ), Material Sciences (United States) (US), Centre de Recherche en Technologie des Semi-conducteurs pour l’Energétique (DZ), Université de Rennes (FR)
Affordable and clean energy
Openalex Percentile: Top 22%
Polymer Nanocomposites and Properties
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