Environmental Impacts and Life Cycle Assessment of Recycled Plastic Bricks

Abstract This study evaluated the mechanical performance, contaminant release, and life-cycle impacts of recycled plastic blocks manufactured from beach-collected and facility-sourced plastic waste. Four formulations combining polyethylene terephthalate, high-density polyethylene, low-density polyethylene, sand, and glass were evaluated. Unweathered blocks had compressive strengths between 20.6–24.3 N/mm2, suitable for paving applications; however, higher plastic fractions led to lower strength and higher porosity. UV weathering reduced strength by 6–12% and increased metal leaching by up to ∼400%. Per- and polyfluorinated concentrations peaked at 13.8 ng/L; concentrations decreased slightly after weathering due to polymer photo-oxidation and embrittlement that enhanced sorption capacity and retention. Formulations with lower plastic content (∼33%) had higher strength and lower leaching. Life-cycle assessment identified extrusion and waste-plastic processing as dominant contributors to climate change (0.12 kg CO2-eq/kg block) and particulate matter (0.42 x 10–3 kg PM10-eq/kg block), driven by fossil-based energy use and process emissions. Blocks with higher plastic ratios exhibited greater environmental burdens, matching leaching trends. These findings revealed that incorporating waste plastics into construction materials can support waste management and infrastructure, but durability, contaminant release, and processing emissions are sensitive to the formulation. Optimizing plastic-to-aggregate ratios and improving processing efficiency can improve durability while reducing environmental and health risks.

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Publication Details

Journal
ACS Omega
Published
2026-09-08
DOI
https://doi.org/10.1021/acsomega.6c04677
Primary Topic
Microplastics and Plastic Pollution
Type
article
Field-Weighted Citation Impact
0.00

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article

Environmental Impacts and Life Cycle Assessment of Recycled Plastic Bricks

Sumanta Das, Bradley O. Clarke, Rainer Lohmann, Šimon Vojta et al.
ACS Omega
Microplastics and Plastic Pollution
article

Environmental Impacts and Life Cycle Assessment of Recycled Plastic Bricks

Sumanta Das, Bradley O. Clarke, Rainer Lohmann, Šimon Vojta, Rakesh Paswan, Jitka Bečanová, Rui Wang, Sirri Neba Nforsoh, Marlene Prien, Karla Pozo, Vinka Oyanedel-Craver, Kayla Kurtz
article en

Abstract

Abstract This study evaluated the mechanical performance, contaminant release, and life-cycle impacts of recycled plastic blocks manufactured from beach-collected and facility-sourced plastic waste. Four formulations combining polyethylene terephthalate, high-density polyethylene, low-density polyethylene, sand, and glass were evaluated. Unweathered blocks had compressive strengths between 20.6–24.3 N/mm2, suitable for paving applications; however, higher plastic fractions led to lower strength and higher porosity. UV weathering reduced strength by 6–12% and increased metal leaching by up to ∼400%. Per- and polyfluorinated concentrations peaked at 13.8 ng/L; concentrations decreased slightly after weathering due to polymer photo-oxidation and embrittlement that enhanced sorption capacity and retention. Formulations with lower plastic content (∼33%) had higher strength and lower leaching. Life-cycle assessment identified extrusion and waste-plastic processing as dominant contributors to climate change (0.12 kg CO2-eq/kg block) and particulate matter (0.42 x 10–3 kg PM10-eq/kg block), driven by fossil-based energy use and process emissions. Blocks with higher plastic ratios exhibited greater environmental burdens, matching leaching trends. These findings revealed that incorporating waste plastics into construction materials can support waste management and infrastructure, but durability, contaminant release, and processing emissions are sensitive to the formulation. Optimizing plastic-to-aggregate ratios and improving processing efficiency can improve durability while reducing environmental and health risks.

ACS Omega
The University of Melbourne (AU), University of Rhode Island (US), Masaryk University (CZ), San Sebastián University (CL), RECETOX (CZ)
National Science Foundation, University of Rhode Island, Rhode Island College, National Oceanic and Atmospheric Administration, Office of Integrative Activities, Office of Experimental Program to Stimulate Competitive Research
Responsible consumption and production
Openalex Percentile: Top 21%
Microplastics and Plastic Pollution
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