Twist-induced chiral phonon coupling in carbon nanotubes from nonlinear elasticity

Twisted carbon nanotubes support phonons involving not only torsion, naturally associated with microrotation, but also radial breathing, which requires a scalar stretch degree of freedom. We derive an effective microstretch theory for these modes starting from nonlinear elasticity on a cylindrical surface. By linearizing the equation of motion around a uniformly twisted equilibrium configuration, we obtain the dynamical matrix for the twisting, longitudinal, and radial-breathing modes. This matrix coincides with that of a one-dimensional microstretch theory, and the corresponding elastic constants are expressed in terms of the Lamé constants, the nanotube radius, and the twist rate. The twist generates chiral couplings in the effective theory, which hybridize the three modes and open an anticrossing in the phonon dispersion. We also discuss the relation between this twist-induced mechanism and intrinsic chirality in chiral nanotubes, where symmetry allows analogous effective chiral couplings even without an externally applied twist. These results provide a microscopic basis for the microstretch description of phonons in twisted carbon nanotubes and clarify how structural chirality enters the effective couplings.

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Publication Details

Journal
Journal of Physics Condensed Matter
Published
2026-08-28
DOI
https://doi.org/10.1088/1361-648x/aea049
Primary Topic
Carbon Nanotubes in Composites
Type
article
Field-Weighted Citation Impact
0.00

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article

Twist-induced chiral phonon coupling in carbon nanotubes from nonlinear elasticity

Takeo Kato, Naoki Nishimura, Mamoru Matsuo
Journal of Physics Condensed Matter
Carbon Nanotubes in Composites
article

Twist-induced chiral phonon coupling in carbon nanotubes from nonlinear elasticity

Takeo Kato, Naoki Nishimura, Mamoru Matsuo
article en

Abstract

Twisted carbon nanotubes support phonons involving not only torsion, naturally associated with microrotation, but also radial breathing, which requires a scalar stretch degree of freedom. We derive an effective microstretch theory for these modes starting from nonlinear elasticity on a cylindrical surface. By linearizing the equation of motion around a uniformly twisted equilibrium configuration, we obtain the dynamical matrix for the twisting, longitudinal, and radial-breathing modes. This matrix coincides with that of a one-dimensional microstretch theory, and the corresponding elastic constants are expressed in terms of the Lamé constants, the nanotube radius, and the twist rate. The twist generates chiral couplings in the effective theory, which hybridize the three modes and open an anticrossing in the phonon dispersion. We also discuss the relation between this twist-induced mechanism and intrinsic chirality in chiral nanotubes, where symmetry allows analogous effective chiral couplings even without an externally applied twist. These results provide a microscopic basis for the microstretch description of phonons in twisted carbon nanotubes and clarify how structural chirality enters the effective couplings.

Journal of Physics Condensed Matter
Kavli Institute for Theoretical Sciences (CN), Institute for Solid State Physics and Optics (HU), The University of Tokyo (JP)
National Natural Science Foundation of China
Peace, Justice and strong institutions
Openalex Percentile: Top 23%
Carbon Nanotubes in Composites
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Twist-induced chiral phonon coupling in carbon nanotubes from nonlinear elasticity — Takeo Kato, Naoki Nishimura, et al. · Journal of Physics Condensed Matter (2026) | TGRS Research Map | TGRS