Neural Network Driven by Electrochemical Performance Data for Predicting the Discharge Termination Time of Seawater Electrolyte-Based Metal-Air Batteries

Seawater electrolyte-based metal-air batteries exhibit great promise for marine energy supply systems. However, conventional statistical analysis methods, though applicable to seawater metal-air battery lifetime prediction, have inherent limitations of insufficient prediction accuracy and large error. Herein, a deep time-series regression framework based on InceptionTime and incorporating prior-biased attention pooling is proposed to construct a nonlinear mapping between electrochemical performance sequences and the discharge termination time of catalysts. Specifically, chronoamperometric profiles are employed to extract long-term stability features, while prior knowledge derived from linear sweep voltammetry is introduced to strengthen the attention weighting over critical potential regions. Under a nested leave-one-catalyst-out cross-validation framework with the one-standard-error rule for epoch selection, the model demonstrates high consistency across various aggregation strategies on a small-sample test set containing different air cathode catalysts, yielding a coefficient of determination over 0.90. These findings suggest that integrating multiscale temporal features with electrochemical prior knowledge through an attention-driven regression framework can improve the prediction accuracy and reduce the prediction error of discharge termination time in the current dataset, thereby providing a preliminary data-driven approach for catalyst evaluation in seawater metal-air batteries.

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Publication Details

Journal
Journal of Electrochemistry
Published
2026-08-28
DOI
https://doi.org/10.61558/2993-074x.3616
Primary Topic
Machine Learning in Materials Science
Type
article
Field-Weighted Citation Impact
0.00

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article

Neural Network Driven by Electrochemical Performance Data for Predicting the Discharge Termination Time of Seawater Electrolyte-Based Metal-Air Batteries

Yu‐Rong Liu, Peng Rao, Yi-Chi Pan, Ning Niu et al.
Journal of Electrochemistry
Machine Learning in Materials Science
article

Neural Network Driven by Electrochemical Performance Data for Predicting the Discharge Termination Time of Seawater Electrolyte-Based Metal-Air Batteries

Yu‐Rong Liu, Peng Rao, Yi-Chi Pan, Ning Niu, Xin-Long Tian, Peng-Peng Shen, De-Kun Yang, Lu-Dan Zhang, Guan-Jun Wang
article en

Abstract

Seawater electrolyte-based metal-air batteries exhibit great promise for marine energy supply systems. However, conventional statistical analysis methods, though applicable to seawater metal-air battery lifetime prediction, have inherent limitations of insufficient prediction accuracy and large error. Herein, a deep time-series regression framework based on InceptionTime and incorporating prior-biased attention pooling is proposed to construct a nonlinear mapping between electrochemical performance sequences and the discharge termination time of catalysts. Specifically, chronoamperometric profiles are employed to extract long-term stability features, while prior knowledge derived from linear sweep voltammetry is introduced to strengthen the attention weighting over critical potential regions. Under a nested leave-one-catalyst-out cross-validation framework with the one-standard-error rule for epoch selection, the model demonstrates high consistency across various aggregation strategies on a small-sample test set containing different air cathode catalysts, yielding a coefficient of determination over 0.90. These findings suggest that integrating multiscale temporal features with electrochemical prior knowledge through an attention-driven regression framework can improve the prediction accuracy and reduce the prediction error of discharge termination time in the current dataset, thereby providing a preliminary data-driven approach for catalyst evaluation in seawater metal-air batteries.

Journal of ElectrochemistryVol. 32(8)
Hainan University (CN), Hainan Agricultural School (CN)
National Natural Science Foundation of China, Hainan University
Openalex Percentile: Top 23%
Machine Learning in Materials Science
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