Enhanced thermal conductivity in natural graphite-based multigraphene materials

We report natural graphite-based multigraphene materials with thermal conductivity enhanced by 20% compared to our previously reported results. The influence of density on the thermal conductivity of these materials was examined. Increasing the density from 1.0 to 1.8 g cm−3 leads to a more than twofold enhancement in thermal conductivity, surpassing the 600 W m−1 K−1 threshold. This result is attributed to a reduction in crystallite misorientation angles to below 15° and a two-order-of-magnitude decrease in defect density from 2 × 10−2 % to 4 × 10−4 %. A multiscale thermal conductivity model for such multigraphene materials was developed, calibrated, and assessed using experimental x-ray diffraction data and electrical conductivity measurements.

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Publication Details

Journal
Applied Physics Letters
Published
2026-08-17
DOI
https://doi.org/10.1063/5.0343403
Primary Topic
Thermal properties of materials
Type
article
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article

Enhanced thermal conductivity in natural graphite-based multigraphene materials

Vladimir A. Shulyak, K. K. Abgaryan, Н. С. Морозов, Kristina E. Klyukova et al.
Applied Physics Letters
Thermal properties of materials
article

Enhanced thermal conductivity in natural graphite-based multigraphene materials

Vladimir A. Shulyak, K. K. Abgaryan, Н. С. Морозов, Kristina E. Klyukova, Victor Vasil’evich Avdeev, Sergei N. Chebotarev, A. A. Zhuravlev, Alexandra V. Gracheva, V. Yu. Gubin, M. G. Morozov, I. K. Nigmatullin, A. N. Silyutin
article en

Abstract

We report natural graphite-based multigraphene materials with thermal conductivity enhanced by 20% compared to our previously reported results. The influence of density on the thermal conductivity of these materials was examined. Increasing the density from 1.0 to 1.8 g cm−3 leads to a more than twofold enhancement in thermal conductivity, surpassing the 600 W m−1 K−1 threshold. This result is attributed to a reduction in crystallite misorientation angles to below 15° and a two-order-of-magnitude decrease in defect density from 2 × 10−2 % to 4 × 10−4 %. A multiscale thermal conductivity model for such multigraphene materials was developed, calibrated, and assessed using experimental x-ray diffraction data and electrical conductivity measurements.

Applied Physics LettersVol. 129(7)
Lomonosov Moscow State University (RU), Moscow State University (TJ)
Openalex Percentile: Top 21%
Thermal properties of materials
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