Demonstrating the accuracy of terahertz absorption spectroscopy and cavity ringdown spectroscopy by a comparison of atomic oxygen density measurements

This work presents a comparison of absolute ground-state atomic oxygen densities measured with terahertz (THz) absorption spectroscopy and cavity ringdown spectroscopy (CRDS). All measurements were performed on the same capacitively coupled radio frequency oxygen discharge, for applied powers in the range of 20–100 W and gas pressures of 70 and 130 Pa. When preconditioning of the reactor walls was taken into account to ensure reproducibility of the results, the atomic oxygen densities obtained with THz absorption spectroscopy and CRDS were found to be in excellent agreement. It can be concluded that both of these techniques can be reliably used to measure line-of-sight integrated atomic oxygen densities with high accuracy.

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Publication Details

Journal
Journal of Applied Physics
Published
2026-08-18
DOI
https://doi.org/10.1063/5.0341443
Primary Topic
Spectroscopy and Laser Applications
Type
article
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article

Demonstrating the accuracy of terahertz absorption spectroscopy and cavity ringdown spectroscopy by a comparison of atomic oxygen density measurements

J. H. van Helden, Klaus‐Dieter Weltmann, Uwe Macherius, Kristaq Gazeli et al.
Journal of Applied Physics
Spectroscopy and Laser Applications
article

Demonstrating the accuracy of terahertz absorption spectroscopy and cavity ringdown spectroscopy by a comparison of atomic oxygen density measurements

J. H. van Helden, Klaus‐Dieter Weltmann, Uwe Macherius, Kristaq Gazeli, Laurent Invernizzi, Jente R. Wubs, A S C Nave, L. Schrottke, G. Lombardi, Xiang Lü
article en

Abstract

This work presents a comparison of absolute ground-state atomic oxygen densities measured with terahertz (THz) absorption spectroscopy and cavity ringdown spectroscopy (CRDS). All measurements were performed on the same capacitively coupled radio frequency oxygen discharge, for applied powers in the range of 20–100 W and gas pressures of 70 and 130 Pa. When preconditioning of the reactor walls was taken into account to ensure reproducibility of the results, the atomic oxygen densities obtained with THz absorption spectroscopy and CRDS were found to be in excellent agreement. It can be concluded that both of these techniques can be reliably used to measure line-of-sight integrated atomic oxygen densities with high accuracy.

Journal of Applied PhysicsVol. 140(7)
Centre National de la Recherche Scientifique (FR), Sorbonne Université (FR), Leibniz Institute for Plasma Science and Technology (DE), Université Sorbonne Paris Nord (FR), Laboratoire des Sciences des Procédés et des Matériaux (FR), Silicon Austria Labs (Austria) (AT), Forschungsverbund Berlin (DE), Eindhoven University of Technology (NL), Ruhr University Bochum (DE)
Openalex Percentile: Top 19%
Spectroscopy and Laser Applications
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