Density-selected topological pathways in the melting of single-particle-thick stripes

The melting of stripe-forming systems involves changes in connectivity that are not fully captured by conventional structural and orientational descriptors. We investigate a two-dimensional model with competing interactions whose low-temperature phase consists of one-particle-thick stripes. Molecular dynamics simulations along seven heating isochores are analyzed using thermodynamic, orientational, dynamical, and graph-based observables. Heating produces a multistage reconstruction in which the loss of stripe alignment and the reorganization of filament connectivity occur over distinct temperature ranges. Density controls whether the disordered filaments fragment into finite polymer-like clusters or remain joined in a dynamically fluid, system-spanning network. The topological observables distinguish these outcomes, which are not resolved by the thermodynamic and orientational responses alone. Thus, the same ordered stripe microphase can melt into topologically distinct fluids selected by density.

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Publication Details

Journal
Physical review. E
Published
2026-10-14
DOI
https://doi.org/10.1103/w3lf-h7nt
Primary Topic
Material Dynamics and Properties
Type
article
Field-Weighted Citation Impact
0.00

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article

Density-selected topological pathways in the melting of single-particle-thick stripes

José Rafael Bordin
Physical review. E
Material Dynamics and Properties
article

Density-selected topological pathways in the melting of single-particle-thick stripes

José Rafael Bordin
article en

Abstract

The melting of stripe-forming systems involves changes in connectivity that are not fully captured by conventional structural and orientational descriptors. We investigate a two-dimensional model with competing interactions whose low-temperature phase consists of one-particle-thick stripes. Molecular dynamics simulations along seven heating isochores are analyzed using thermodynamic, orientational, dynamical, and graph-based observables. Heating produces a multistage reconstruction in which the loss of stripe alignment and the reorganization of filament connectivity occur over distinct temperature ranges. Density controls whether the disordered filaments fragment into finite polymer-like clusters or remain joined in a dynamically fluid, system-spanning network. The topological observables distinguish these outcomes, which are not resolved by the thermodynamic and orientational responses alone. Thus, the same ordered stripe microphase can melt into topologically distinct fluids selected by density.

Physical review. E
Alexander von Humboldt-Stiftung, Coordenação de Aperfeiçoamento de Pessoal de Nível Superior, Conselho Nacional de Desenvolvimento Científico e Tecnológico, Fundação de Amparo à Pesquisa do Estado do Rio Grande do Sul, Universität Konstanz
Openalex Percentile: Top 50%
Material Dynamics and Properties
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