Monolayer <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>MnBi</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi>Te</mml:mi> <mml:mn>4</mml:mn> </mml:msub> </mml:mrow> </mml:math> : Atomic-scale insigh
As the first intrinsic antiferromagnetic topological insulator, ${\mathrm{MnBi}}_{2}{\mathrm{Te}}_{4}$ offers a platform for investigating topological phenomena driven by magnetism. Prior studies focused on bulk single crystals and exfoliated flakes, but the extreme two-dimensional (2D) limit remains underexplored, despite theoretical predictions of exotic behavior. In particular, synthesis and atomic-scale characterization of ultrathin ${\mathrm{MnBi}}_{2}{\mathrm{Te}}_{4}$ films remain challenging. Here we explore molecular beam epitaxy grown ${\mathrm{MnBi}}_{2}{\mathrm{Te}}_{4}$ thin films down to a single-layer thickness. Structural characterization via electron and x-ray diffraction, atomic force microscopy, and scanning tunneling microscopy confirms layer-by-layer growth and high crystallinity, while magnetotransport measurements show the expected magnetic signatures. Interestingly, scanning tunneling microscopy and quasiparticle interference imaging reveal Dirac-like surface states that persist even in monolayer films and monolayer islands. Our experiments provide elusive atomic-scale insights into the band structure of ${\mathrm{MnBi}}_{2}{\mathrm{Te}}_{4}$ in the 2D limit and under lateral confinement, and establish a foundation for the synthesis of heterostructures based on monolayer ${\mathrm{MnBi}}_{2}{\mathrm{Te}}_{4}$ and device applications.
Authors
- Hengxin Tan (ORCID: https://orcid.org/0000-0002-6366-4731)
- Ilija Zeljkovic (ORCID: https://orcid.org/0000-0001-9966-2140)
- Binghai Yan (ORCID: https://orcid.org/0000-0003-2164-5839)
- Alexander LaFleur
- Siyuan Ding (ORCID: https://orcid.org/0000-0001-6813-7271)
- Vsevolod Belosevich (ORCID: https://orcid.org/0000-0001-9122-4920)
- Wilber Alfaro Castro (ORCID: https://orcid.org/0009-0007-8527-923X)
- Zumeng Huang (ORCID: https://orcid.org/0009-0000-7046-276X)
- Qiong Ma (ORCID: https://orcid.org/0000-0002-5103-6973)
- Muxian Xu
Institutions
- Boston College (US)
- Pennsylvania State University (US)
- Shanghai Jiao Tong University (CN)
Publication Details
- Journal
- Physical Review Materials
- Published
- 2026-07-27
- DOI
- https://doi.org/10.1103/zmzs-krb9
- Primary Topic
- Topological Materials and Phenomena
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- U.S. Department of Energy