Mapping CO2 migration pathways: interactions with geological structures

Unintended CO2 releases from carbon capture and storage sites could impact water resources or reverse climate mitigation efforts through atmospheric emissions. Comprehensive understanding of how CO2 migrates in the shallow subsurface is required for appropriate monitoring of any CO2 release. Here, 3D metre-scale realistic sedimentary bedforms were generated to represent a variety of cross-bedding structures with varied contrasts between the grain size of the bedding and lamina. Gas migration simulations were conducted through each sedimentary structure, demonstrating the sensitivity of gas migration to centimetre-scale bedding structures. A bedding-laminae grain size contrast threshold was identified at which mass distributions transition from ganglia-dominated to pool-dominated. Furthermore, this threshold coincides with a transition from vertically-dominated to horizontally-dominated flow, regardless of bedding structure. This indicates that centimetre-scale heterogeneity could prevent gas reaching the surface in the event of a release, but simultaneously cause unanticipated lateral migration away from the release site.

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Publication Details

Journal
Edinburgh Research Explorer (University of Edinburgh)
Published
2026-07-28
DOI
https://doi.org/10.1029/2025gl119210digital
Primary Topic
CO2 Sequestration and Geologic Interactions
Type
article
Field-Weighted Citation Impact
0.00

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article

Mapping CO2 migration pathways: interactions with geological structures

Stuart; id_orcid 0000-0003-1929-2843 Gilfillan, Ian; id_orcid 0000-0002-6610-4975 Molnar, Magdalena Krol, Nicholas; id_orcid 0000-0001-6491-7078 Ashmore
Edinburgh Research Explorer (University of Edinburgh)
CO2 Sequestration and Geologic Interactions
article

Mapping CO2 migration pathways: interactions with geological structures

Stuart; id_orcid 0000-0003-1929-2843 Gilfillan, Ian; id_orcid 0000-0002-6610-4975 Molnar, Magdalena Krol, Nicholas; id_orcid 0000-0001-6491-7078 Ashmore
article en

Abstract

Unintended CO2 releases from carbon capture and storage sites could impact water resources or reverse climate mitigation efforts through atmospheric emissions. Comprehensive understanding of how CO2 migrates in the shallow subsurface is required for appropriate monitoring of any CO2 release. Here, 3D metre-scale realistic sedimentary bedforms were generated to represent a variety of cross-bedding structures with varied contrasts between the grain size of the bedding and lamina. Gas migration simulations were conducted through each sedimentary structure, demonstrating the sensitivity of gas migration to centimetre-scale bedding structures. A bedding-laminae grain size contrast threshold was identified at which mass distributions transition from ganglia-dominated to pool-dominated. Furthermore, this threshold coincides with a transition from vertically-dominated to horizontally-dominated flow, regardless of bedding structure. This indicates that centimetre-scale heterogeneity could prevent gas reaching the surface in the event of a release, but simultaneously cause unanticipated lateral migration away from the release site.

Edinburgh Research Explorer (University of Edinburgh)
Natural Environment Research Council
Clean water and sanitation
Openalex Percentile: Top 22%
CO2 Sequestration and Geologic Interactions
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