Nonperturbative nonlinear Hall effect in nonequilibrium steady states

The nonlinear Hall effect in quantum materials has attracted broad interest, yet most existing studies focus on the weak-field, perturbative regime. Here we develop a nonperturbative approach based on nonequilibrium steady-state Green's functions for dc-field-driven lattice systems, with dissipation and interactions incorporated through self-energies beyond the constant relaxation-time approximation and interband transitions treated alongside their intraband counterparts. Applied to a two-band semimetal model, our approach provides direct access to the strong-field Hall response beyond the nonperturbative crossover where the edge of the nonequilibrium distribution reaches Berry-curvature hot spots, a regime in which constant relaxation-time estimates and Berry curvature dipole calculations become unreliable. We further demonstrate that interaction and electron-phonon self-energies within dynamical mean-field theory can substantially change the Hall signal. Our framework enables quantitative simulations of nonequilibrium nonlinear Hall phenomena and provides guidance for strong-field transport experiments.

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Publication Details

Journal
Physical Review Letters
Published
2026-10-14
DOI
https://doi.org/10.1103/dy42-1yz7
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
0.00

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article

Nonperturbative nonlinear Hall effect in nonequilibrium steady states

Silke Buehler Paschen, Shouvik Sur, Qimiao Si A, MARTIN C. ECKSTEIN et al.
Physical Review Letters
Topological Materials and Phenomena
article

Nonperturbative nonlinear Hall effect in nonequilibrium steady states

Silke Buehler Paschen, Shouvik Sur, Qimiao Si A, MARTIN C. ECKSTEIN, Philipp Werner, Lei Geng, Lei Chen
article en

Abstract

The nonlinear Hall effect in quantum materials has attracted broad interest, yet most existing studies focus on the weak-field, perturbative regime. Here we develop a nonperturbative approach based on nonequilibrium steady-state Green's functions for dc-field-driven lattice systems, with dissipation and interactions incorporated through self-energies beyond the constant relaxation-time approximation and interband transitions treated alongside their intraband counterparts. Applied to a two-band semimetal model, our approach provides direct access to the strong-field Hall response beyond the nonperturbative crossover where the edge of the nonequilibrium distribution reaches Berry-curvature hot spots, a regime in which constant relaxation-time estimates and Berry curvature dipole calculations become unreliable. We further demonstrate that interaction and electron-phonon self-energies within dynamical mean-field theory can substantially change the Hall signal. Our framework enables quantitative simulations of nonequilibrium nonlinear Hall phenomena and provides guidance for strong-field transport experiments.

Physical Review Letters
National Science Foundation, Aspen Center for Physics, Rice University, Deutsche Forschungsgemeinschaft, Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung, Austrian Science Fund, Université de Fribourg, National Center of Competence in Research Materials’ Revolution: Computational Design and Discovery of Novel Materials, Office of Naval Research, Division of Materials Research
Openalex Percentile: Top 52%
Topological Materials and Phenomena
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