From Tracks to Hotspots: Particle-Dependent Radiation Energy Deposition in MAPbI3 Perovskite

Geant4 (version 11.3.2) simulations were used to study particle-dependent radiation interaction in MAPbI3 under electron, photon, and neutron irradiation. The analysis focused on spatial distributions of interaction events, released energy, secondary-particle generation, and process-specific contributions. A 1 mm single-layer MAPbI3 target was used to identify the intrinsic material response, while multilayer MAPbI3 containing detector geometries were considered to assess device-like effects. Electrons produced extended charged particle tracks governed by direct energy loss and secondary-electron cascades. Photons showed weak direct energy deposition, with the response mainly controlled by secondary electrons generated in discrete electromagnetic interactions. Neutrons produced sparse but locally intense energy-release patterns dominated by recoil particles and nuclear-reaction products. The results show that total released energy alone is insufficient to describe radiation response in MAPbI3; spatial morphology and the balance between primary and secondary contributions are essential for interpreting both detector operation and possible radiation-induced degradation.

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Publication Details

Journal
Nanomaterials
Published
2026-06-29
DOI
https://doi.org/10.3390/nano16130803
Primary Topic
Perovskite Materials and Applications
Type
article
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article

From Tracks to Hotspots: Particle-Dependent Radiation Energy Deposition in MAPbI3 Perovskite

Huiliang Sun, Ivan S. Zhidkov, Ivan E. Novoselov, Zhi Xing
Nanomaterials
Perovskite Materials and Applications
article

From Tracks to Hotspots: Particle-Dependent Radiation Energy Deposition in MAPbI3 Perovskite

Huiliang Sun, Ivan S. Zhidkov, Ivan E. Novoselov, Zhi Xing
article en

Abstract

Geant4 (version 11.3.2) simulations were used to study particle-dependent radiation interaction in MAPbI3 under electron, photon, and neutron irradiation. The analysis focused on spatial distributions of interaction events, released energy, secondary-particle generation, and process-specific contributions. A 1 mm single-layer MAPbI3 target was used to identify the intrinsic material response, while multilayer MAPbI3 containing detector geometries were considered to assess device-like effects. Electrons produced extended charged particle tracks governed by direct energy loss and secondary-electron cascades. Photons showed weak direct energy deposition, with the response mainly controlled by secondary electrons generated in discrete electromagnetic interactions. Neutrons produced sparse but locally intense energy-release patterns dominated by recoil particles and nuclear-reaction products. The results show that total released energy alone is insufficient to describe radiation response in MAPbI3; spatial morphology and the balance between primary and secondary contributions are essential for interpreting both detector operation and possible radiation-induced degradation.

NanomaterialsVol. 16(13)
Ural Federal University (RU), Guangzhou University (CN), M.N. Mikheev Institute of Metal Physics (RU), Institute of Problems of Chemical Physics (RU), Gannan Normal University (CN)
Affordable and clean energy
Openalex Percentile: Top 11%
Perovskite Materials and Applications
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