Observation-constrained sensitivities of Arctic methane emissions to warming
The sensitivity of pan-Arctic (60 to 90°N) natural methane emissions to climate warming lacks direct observational constraints. Long-term atmospheric measurements of methane, which reflect integrated Arctic fluxes and atmospheric transport, show that in the pan-Arctic the autumn-to-winter CH 4 build-up (as indicated by the “autumn zero crossing date”) is becoming earlier. This advancing trend in autumn zero crossing date is explained by growing natural Arctic CH 4 emissions in response to climate warming in July, August and September, with a rate of increase of 0.14 ± 0.04 Tg CH 4 y −2 during the period 1998–2020. Atmospheric δ 13 C CH4 observational records allowed us to attribute this increase to 0.08 ± 0.02 Tg CH 4 y −2 from natural biogenic emissions (wetlands, lakes, permafrost soils) and 0.06 ± 0.02 Tg CH 4 y −2 from wildfire emissions. Our results point to a larger warming sensitivity of natural emissions (3.1 ± 0.9 Tg CH 4 y −1 per °C) than previous estimates, and potentially a larger positive feedback on climate warming.
Authors
- Shushi Peng (ORCID: https://orcid.org/0000-0001-5098-726X)
- Gang Liu (ORCID: https://orcid.org/0000-0002-7613-1985)
- Lu Shen (ORCID: https://orcid.org/0000-0003-2787-7016)
- Euan G. Nisbet (ORCID: https://orcid.org/0000-0001-8379-857X)
- Sylvia Michel (ORCID: https://orcid.org/0000-0002-5651-1163)
- Philippe Ciais (ORCID: https://orcid.org/0000-0001-8560-4943)
- Xin Lan
Institutions
- National Oceanic and Atmospheric Administration (US)
- Cooperative Institute for Research in Environmental Sciences (US)
- Institute of Arctic and Alpine Research (US)
- Royal Holloway University of London (GB)
- Peking University (CN)
- Commissariat à l'Énergie Atomique et aux Énergies Alternatives (FR)
- Université Paris-Saclay (FR)
- NOAA Oceanic and Atmospheric Research (US)
- Earth Science Institute of the Slovak Academy of Sciences (SK)
Publication Details
- Journal
- Proceedings of the National Academy of Sciences
- Published
- 2026-06-29
- DOI
- https://doi.org/10.1073/pnas.2523274123
- Primary Topic
- Atmospheric and Environmental Gas Dynamics
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- National Natural Science Foundation of China
- Yunnan Provincial Science and Technology Department