Anthropogenic modulation of dust-dominated ice nucleation in an urban dryland city of China during winter and spring
Abstract. Ice-nucleating particles (INPs) are crucial for cloud and precipitation modulation, yet their spatiotemporal variability and sources sampled from urban dryland regions remain poorly understood. While natural dust is recognized as a substantial source of INPs, its interaction and quantity with anthropogenic pollutants, as well as INP abundance of the mixtures, remain insufficiently quantified. Here, we present online observations of INPs (−15 to −35 °C), together with co-located aerosol size distribution and chemical composition in Lanzhou from winter 2024 to spring 2025. We show that long-range dust transport boosts INP concentrations by a factor of 15 at −30 °C in an urban region. Elevated secondary inorganic aerosol was observed during winter pollution events and negatively correlated with INP activity (R = −0.71). We further refine an INP parameterization based on aerosol size (1–2.5 µm) and freezing temperature, reproducing 83 % of observations within a factor of 5. These findings underscore the need to include local aerosol heterogeneity and dust-pollution interactions in INP parameterizations for more accurate regional climate simulations.
Authors
- Lu Feng
- Yue Wang (ORCID: https://orcid.org/0000-0003-0098-5359)
- Jiming Li (ORCID: https://orcid.org/0000-0002-7286-3580)
- Yi-Xiang Wang (ORCID: https://orcid.org/0000-0002-5246-5497)
- Chengqing Chen (ORCID: https://orcid.org/0009-0002-4619-6830)
- Tianrong Chai
- Zhao Ji
Institutions
- Nanjing Institute of Technology (CN)
- Lanzhou University (CN)
Publication Details
- Journal
- Atmospheric chemistry and physics
- Published
- 2026-06-26
- DOI
- https://doi.org/10.5194/acp-26-9017-2026
- Primary Topic
- Atmospheric aerosols and clouds
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Innovative Research Group Project of the National Natural Science Foundation of China
- National Natural Science Foundation of China
- Science and Technology Department of Gansu Province
- Fundamental Research Funds for the Central Universities