Anthropogenic modulation of dust-dominated ice nucleation in an urban dryland city of China during winter and spring

Abstract. Ice-nucleating particles (INPs) are crucial for cloud and precipitation modulation, yet their spatiotemporal variability and sources sampled from urban dryland regions remain poorly understood. While natural dust is recognized as a substantial source of INPs, its interaction and quantity with anthropogenic pollutants, as well as INP abundance of the mixtures, remain insufficiently quantified. Here, we present online observations of INPs (−15 to −35 °C), together with co-located aerosol size distribution and chemical composition in Lanzhou from winter 2024 to spring 2025. We show that long-range dust transport boosts INP concentrations by a factor of 15 at −30 °C in an urban region. Elevated secondary inorganic aerosol was observed during winter pollution events and negatively correlated with INP activity (R = −0.71). We further refine an INP parameterization based on aerosol size (1–2.5 µm) and freezing temperature, reproducing 83 % of observations within a factor of 5. These findings underscore the need to include local aerosol heterogeneity and dust-pollution interactions in INP parameterizations for more accurate regional climate simulations.

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Publication Details

Journal
Atmospheric chemistry and physics
Published
2026-06-26
DOI
https://doi.org/10.5194/acp-26-9017-2026
Primary Topic
Atmospheric aerosols and clouds
Type
article
Field-Weighted Citation Impact
0.00

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article

Anthropogenic modulation of dust-dominated ice nucleation in an urban dryland city of China during winter and spring

Lu Feng, Yue Wang, Jiming Li, Yi-Xiang Wang et al.
Atmospheric chemistry and physics
Atmospheric aerosols and clouds
article

Anthropogenic modulation of dust-dominated ice nucleation in an urban dryland city of China during winter and spring

Lu Feng, Yue Wang, Jiming Li, Yi-Xiang Wang, Chengqing Chen, Tianrong Chai, Zhao Ji
article en

Abstract

Abstract. Ice-nucleating particles (INPs) are crucial for cloud and precipitation modulation, yet their spatiotemporal variability and sources sampled from urban dryland regions remain poorly understood. While natural dust is recognized as a substantial source of INPs, its interaction and quantity with anthropogenic pollutants, as well as INP abundance of the mixtures, remain insufficiently quantified. Here, we present online observations of INPs (−15 to −35 °C), together with co-located aerosol size distribution and chemical composition in Lanzhou from winter 2024 to spring 2025. We show that long-range dust transport boosts INP concentrations by a factor of 15 at −30 °C in an urban region. Elevated secondary inorganic aerosol was observed during winter pollution events and negatively correlated with INP activity (R = −0.71). We further refine an INP parameterization based on aerosol size (1–2.5 µm) and freezing temperature, reproducing 83 % of observations within a factor of 5. These findings underscore the need to include local aerosol heterogeneity and dust-pollution interactions in INP parameterizations for more accurate regional climate simulations.

Atmospheric chemistry and physicsVol. 26(12)
Nanjing Institute of Technology (CN), Lanzhou University (CN)
Innovative Research Group Project of the National Natural Science Foundation of China, National Natural Science Foundation of China, Science and Technology Department of Gansu Province, Fundamental Research Funds for the Central Universities
Climate action
Openalex Percentile: Top 7%
Atmospheric aerosols and clouds
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