Geometry-Driven Performance Enhancement in h-BN/β-Ga <sub>2</sub> O <sub>3</sub> Heterostructures for Solar-Blind and Polarization-Sensitive Photodetection

Solar-blind ultraviolet photodetectors have attracted increasing interest, yet their performance is often limited by inefficient carrier collection and reliance on complex thin-film growth techniques. In this work, we investigate geometry-driven performance enhancement in h-BN/β-Ga 2 O 3 heterostructures fabricated using mechanically exfoliated β-Ga 2 O 3, offering a simple and cost-effective alternative to epitaxial approaches. The exfoliated β-Ga 2 O 3 devices exhibit a clear photoresponse over a broad spectral range from 200 to 405 nm. By systematically comparing vertical and lateral heterostructure architectures, we demonstrate that device geometry plays a decisive role in determining photodetection behavior. The vertical h-BN/β-Ga 2 O 3 photodetector device exhibits a markedly enhanced solar-blind response, achieving a high responsivity of 96.7 AW –1 and an external quantum efficiency of 52258% at 230 nm, which are substantially higher than those of the lateral heterostructure (5.0 AW –1 and 2317%) and the bare β-Ga 2 O 3 photodetector device (0.29 AW –1 and 135%). In addition, polarization-resolved measurements reveal an anisotropic photoresponse with a dichroic ratio of approximately 2.1 for the vertical configuration. Interfacial potential investigations confirm the presence of a built-in electric field that promotes efficient photocarrier separation. These results highlight geometry design as an effective strategy for realizing high-performance, solar-blind, and polarization-sensitive photodetection using straightforward exfoliation-based heterostructures.

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Publication Details

Journal
ACS Applied Materials & Interfaces
Published
2026-06-16
DOI
https://doi.org/10.1021/acsami.6c06163
Primary Topic
Ga2O3 and related materials
Type
article
Field-Weighted Citation Impact
0.00

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article

Geometry-Driven Performance Enhancement in h-BN/β-Ga 2 O 3 Heterostructures for Solar-Blind and Polarization-Sensitive Photodetection

Yu. Yu. Illarionov, Shrouq H. Aleithan, Muhammad Ajmal, Waqas Ahmad
ACS Applied Materials & Interfaces
Ga2O3 and related materials
article

Geometry-Driven Performance Enhancement in h-BN/β-Ga 2 O 3 Heterostructures for Solar-Blind and Polarization-Sensitive Photodetection

Yu. Yu. Illarionov, Shrouq H. Aleithan, Muhammad Ajmal, Waqas Ahmad
article en

Abstract

Solar-blind ultraviolet photodetectors have attracted increasing interest, yet their performance is often limited by inefficient carrier collection and reliance on complex thin-film growth techniques. In this work, we investigate geometry-driven performance enhancement in h-BN/β-Ga 2 O 3 heterostructures fabricated using mechanically exfoliated β-Ga 2 O 3, offering a simple and cost-effective alternative to epitaxial approaches. The exfoliated β-Ga 2 O 3 devices exhibit a clear photoresponse over a broad spectral range from 200 to 405 nm. By systematically comparing vertical and lateral heterostructure architectures, we demonstrate that device geometry plays a decisive role in determining photodetection behavior. The vertical h-BN/β-Ga 2 O 3 photodetector device exhibits a markedly enhanced solar-blind response, achieving a high responsivity of 96.7 AW –1 and an external quantum efficiency of 52258% at 230 nm, which are substantially higher than those of the lateral heterostructure (5.0 AW –1 and 2317%) and the bare β-Ga 2 O 3 photodetector device (0.29 AW –1 and 135%). In addition, polarization-resolved measurements reveal an anisotropic photoresponse with a dichroic ratio of approximately 2.1 for the vertical configuration. Interfacial potential investigations confirm the presence of a built-in electric field that promotes efficient photocarrier separation. These results highlight geometry design as an effective strategy for realizing high-performance, solar-blind, and polarization-sensitive photodetection using straightforward exfoliation-based heterostructures.

ACS Applied Materials & Interfaces
King Fahd University of Petroleum and Minerals (SA), Southern University of Science and Technology (CN), King Faisal University (SA)
National Natural Science Foundation of China, Deanship of Scientific Research, King Faisal University, Basic and Applied Basic Research Foundation of Guangdong Province
Openalex Percentile: Top 17%
Ga2O3 and related materials
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