Retrieval of Atmospheric Microphysical Parameters Using Triple-Wavelength Lidar: Influencing Factors and Case Studies Under Clean and Lightly Polluted Urban Conditions

To address the limited constraints of ground-based lidar with few channels in retrieving aerosol microphysical parameters in urban atmospheres, this study developed a method to retrieve aerosol volume size distribution and effective radius from a 355/532/1064 nm triple-wavelength elastic-scattering, single-polarization lidar system. The method uses 3β + 2α optical quantities as input constraints, applies Mie scattering theory as the forward model, parameterizes the volume size distribution with B-spline functions, and achieves stable solutions through Tikhonov regularization and cross-validation. To reduce uncertainties in prior parameters, including the complex refractive index, particle size range, and lidar ratio, an optimization strategy based on parameter search, retrieval reconstruction, and error minimization was introduced. Numerical simulations showed that the method reproduced the main features of a bimodal lognormal aerosol volume size distribution with good feasibility and stability. Two case studies further showed fine-mode dominance and decreasing extinction coefficient, depolarization ratio, and effective radius with height under good air quality conditions, but enhanced coarse-mode contribution and effective radius in the upper cloud-influenced layer under lightly polluted conditions, as inferred from the combined variations in RSCS, extinction coefficient, depolarization ratio, and effective radius.