Strain Tuning the Occupation of Candidate Topological Weyl States in W‐Doped MoTe <sub>2</sub>

ABSTRACT Strain‐induced modifications of the electronic structure in ‐ were studied using hard X‐ray angle‐resolved photoemission spectroscopy (HARPES). Partial substitution of Mo with W stabilizes the metastable low‐temperature orthorhombic phase of . Samples were first characterized by angle‐resolved photoemission spectroscopy experiments with soft X‐rays and higher resolution, showing good agreement with ab initio calculations of electronic states related to topology. The modification of the bulk electronic structure due to the applied strain was assessed using operando HARPES. Applying tensile strain along the ‐axis with amplitudes up to 0.34% result in changes in the bulk electronic structure as predicted by previous ab‐initio calculations. In particular, the results demonstrate a strain‐driven depletion of electronic states with heavy masses and high scattering rates, leading to an increase in conductivity. In contrast, tensile strain along the ‐axis results in a significant increase in resistivity, which we confirmed by transport studies.

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Publication Details

Journal
Advanced Science
Published
2026-06-12
DOI
https://doi.org/10.1002/advs.76064
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
0.00

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article

Strain Tuning the Occupation of Candidate Topological Weyl States in W‐Doped MoTe 2

Sofia Michaela Souliou, Mehdi Frachet, Christoph Schlueter, Florian Diekmann et al.
Advanced Science
Topological Materials and Phenomena
article

Strain Tuning the Occupation of Candidate Topological Weyl States in W‐Doped MoTe 2

Sofia Michaela Souliou, Mehdi Frachet, Christoph Schlueter, Florian Diekmann, Yaryna Lytvynenko, H. J. Elmers, Dmytro Kutnyakhov, J. Demšar, Harshit Agarwal, O. Fedchenko, Volkmar Koller, G. Schönhense, Olena Tkach, Michael Merz, Moritz Hoesch, Andrei Gloskovskii, Yuriy Mokrousov, Matthieu Le Tacon, Amon Lanz, Kai Rossnagel, Philipp Rüssmann, Sergii V. Chernov
article en

Abstract

ABSTRACT Strain‐induced modifications of the electronic structure in ‐ were studied using hard X‐ray angle‐resolved photoemission spectroscopy (HARPES). Partial substitution of Mo with W stabilizes the metastable low‐temperature orthorhombic phase of . Samples were first characterized by angle‐resolved photoemission spectroscopy experiments with soft X‐rays and higher resolution, showing good agreement with ab initio calculations of electronic states related to topology. The modification of the bulk electronic structure due to the applied strain was assessed using operando HARPES. Applying tensile strain along the ‐axis with amplitudes up to 0.34% result in changes in the bulk electronic structure as predicted by previous ab‐initio calculations. In particular, the results demonstrate a strain‐driven depletion of electronic states with heavy masses and high scattering rates, leading to an increase in conductivity. In contrast, tensile strain along the ‐axis results in a significant increase in resistivity, which we confirmed by transport studies.

Advanced Science
Karlsruhe Institute of Technology (DE), Goethe University Frankfurt (DE), Centre National de la Recherche Scientifique (FR), Forschungszentrum Jülich (DE), Johannes Gutenberg University Mainz (DE), Sumy State University (UA), Deutsches Elektronen-Synchrotron DESY (DE), Christian-Albrechts-Universität zu Kiel (DE), Jülich Aachen Research Alliance (DE), Institut Néel (FR), Institute of Magnetism (UA), Université Grenoble Alpes (FR)
Deutsche Forschungsgemeinschaft, Bundesministerium für Bildung und Forschung
Openalex Percentile: Top 6%
Topological Materials and Phenomena
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