Time-Resolved Dynamics of Semiconductor Nanolaser via Four-Wave Mixing Gating

High Resolution Image Download MS PowerPoint Slide We experimentally demonstrate the direct time-domain characterization of photonic-crystal nanolasers at telecom wavelengths using a nonlinear optical gating technique based on four-wave mixing. This approach enables the temporal characterization of the ultrafast emission dynamics under short-pulse excitation with a picosecond time resolution. When a weak continuous-wave component is added to the pulsed pump, the emission becomes less sensitive to spontaneous-emission noise, resulting in a significantly reduced buildup time. The difference between purely pulsed and hybrid excitation regimes points to the influence of pulse-to-pulse timing fluctuations. To elucidate this effect, we perform Langevin-based simulations that reproduce the experimentally observed broadening and confirm that time jitter, originating from spontaneous emission noise near threshold, dominates the temporal dispersion. These results establish four-wave mixing gating as a powerful method to probe nanolaser dynamics with picosecond precision.

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Publication Details

Journal
ACS Photonics
Published
2026-06-09
DOI
https://doi.org/10.1021/acsphotonics.6c00195
Primary Topic
Plasmonic and Surface Plasmon Research
Type
article
Field-Weighted Citation Impact
0.00

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article

Time-Resolved Dynamics of Semiconductor Nanolaser via Four-Wave Mixing Gating

Fabrice Raineri, Konstantinos Pantzas, Giuseppe Modica, Guilhem Madiot et al.
ACS Photonics
Plasmonic and Surface Plasmon Research
article

Time-Resolved Dynamics of Semiconductor Nanolaser via Four-Wave Mixing Gating

Fabrice Raineri, Konstantinos Pantzas, Giuseppe Modica, Guilhem Madiot, A. M. Yacomotti, Federico Monti, Isabelle Sagnes, Grégoire Beaudoin
article en

Abstract

High Resolution Image Download MS PowerPoint Slide We experimentally demonstrate the direct time-domain characterization of photonic-crystal nanolasers at telecom wavelengths using a nonlinear optical gating technique based on four-wave mixing. This approach enables the temporal characterization of the ultrafast emission dynamics under short-pulse excitation with a picosecond time resolution. When a weak continuous-wave component is added to the pulsed pump, the emission becomes less sensitive to spontaneous-emission noise, resulting in a significantly reduced buildup time. The difference between purely pulsed and hybrid excitation regimes points to the influence of pulse-to-pulse timing fluctuations. To elucidate this effect, we perform Langevin-based simulations that reproduce the experimentally observed broadening and confirm that time jitter, originating from spontaneous emission noise near threshold, dominates the temporal dispersion. These results establish four-wave mixing gating as a powerful method to probe nanolaser dynamics with picosecond precision.

ACS Photonics
Centre National de la Recherche Scientifique (FR), Université Paris-Saclay (FR), Centre de Nanosciences et de Nanotechnologies (FR), Laboratoire Photonique, Numérique et Nanosciences (FR), Institut de Physique de Nice (FR)
Agence Nationale de la Recherche
Affordable and clean energy
Openalex Percentile: Top 11%
Plasmonic and Surface Plasmon Research
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Time-Resolved Dynamics of Semiconductor Nanolaser via Four-Wave Mixing Gating — Fabrice Raineri, Konstantinos Pantzas, et al. · ACS Photonics (2026) | TGRS Research Map | TGRS