N-component free energy lattice Boltzmann method with reduction consistency and global momentum conservation

We present a free energy lattice Boltzmann model capable, in principle, of simulating fluid systems with an arbitrary number of immiscible components. Our method is strictly reduction consistent, ensuring that absent fluid components do not spontaneously nucleate. We introduce a novel discretization of the surface tension force that globally conserves momentum to machine precision, and we enforce reduction consistency through a flux correction that is independent of the mobility. The method is benchmarked with a range of static and dynamic problems, including liquid lenses, Janus droplets, quaternary phase separation, and six-component layered Poiseuille flow, and we obtain excellent agreement with theoretical predictions throughout. Finally, we demonstrate the applicability of the proposed method through patterned liquid surfaces and microfluidic emulsion droplet generation.

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Publication Details

Journal
The Journal of Chemical Physics
Published
2026-06-09
DOI
https://doi.org/10.1063/5.0327062
Primary Topic
Lattice Boltzmann Simulation Studies
Type
article
Field-Weighted Citation Impact
0.00

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article

N-component free energy lattice Boltzmann method with reduction consistency and global momentum conservation

Michael Rennick, Halim Kusumaatmaja, Xitong Zhang, Tim Niklas Bingert et al.
The Journal of Chemical Physics
Lattice Boltzmann Simulation Studies
article

N-component free energy lattice Boltzmann method with reduction consistency and global momentum conservation

Michael Rennick, Halim Kusumaatmaja, Xitong Zhang, Tim Niklas Bingert, Mathias J. Krause
article en

Abstract

We present a free energy lattice Boltzmann model capable, in principle, of simulating fluid systems with an arbitrary number of immiscible components. Our method is strictly reduction consistent, ensuring that absent fluid components do not spontaneously nucleate. We introduce a novel discretization of the surface tension force that globally conserves momentum to machine precision, and we enforce reduction consistency through a flux correction that is independent of the mobility. The method is benchmarked with a range of static and dynamic problems, including liquid lenses, Janus droplets, quaternary phase separation, and six-component layered Poiseuille flow, and we obtain excellent agreement with theoretical predictions throughout. Finally, we demonstrate the applicability of the proposed method through patterned liquid surfaces and microfluidic emulsion droplet generation.

The Journal of Chemical PhysicsVol. 164(22)
Karlsruhe Institute of Technology (DE), University of Edinburgh (GB)
Leverhulme Trust, Deutsche Forschungsgemeinschaft, Engineering and Physical Sciences Research Council
Life in Land
Openalex Percentile: Top 7%
Lattice Boltzmann Simulation Studies
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N-component free energy lattice Boltzmann method with reduction consistency and global momentum conservation — Michael Rennick, Halim Kusumaatmaja, et al. · The Journal of Chemical Physics (2026) | TGRS Research Map | TGRS