Crystallography of periodic nanotextures in a strained Mott insulator
Here we investigate stripes of alternating structural phases spontaneously forming in epitaxially strained $Ca_2RuO_4$ thin films below the metal-insulator transition. Using large-volume X-ray reciprocal-space mapping, we show that satellite-pattern intensities across 24 symmetry-inequivalent Bragg reflections collapse onto a single parameter-free curve. The collapse identifies a coherent martensitic laminate of few-nm-wide domains separated by ${012}$ interfaces, with displacements along $\left\langle01\bar{2}\right\rangle$. Satellite-extinction analysis demonstrates that both coexisting phases retain the bulk orthorhombic space group despite the pseudocubic $LaAlO_3$ substrate, biaxial epitaxial strain, and intrinsic strain at the interfaces. Classical invariant-plane-strain crystallography thus governs the nanoscale domain geometry of a Mott insulator with intertwined magnetic, electronic, and lattice order.
Authors
- Suchismita Sarker (ORCID: https://orcid.org/0000-0002-8820-1143)
- Yorick A. Birkhölzer (ORCID: https://orcid.org/0000-0003-3133-2481)
- Ziming Shao (ORCID: https://orcid.org/0000-0002-4995-277X)
- Noah Schnitzer (ORCID: https://orcid.org/0000-0002-1042-1146)
- Benjamin Z. Gregory
- Andrej Singer (ORCID: https://orcid.org/0000-0002-2965-9242)
- K. M. Shen
- Darrell G. Schlom (ORCID: https://orcid.org/0000-0003-2493-6113)
- Berit Hansen Goodge (ORCID: https://orcid.org/0000-0003-0948-7698)
- Jacob P. Ruff
- Jeffrey W Hodgson
- David A. Muller (ORCID: https://orcid.org/0000-0003-4129-0473)
Publication Details
- Journal
- Physical Review Letters
- Published
- 2026-10-28
- DOI
- https://doi.org/10.1103/kmws-wh4q
- Primary Topic
- Electronic and Structural Properties of Oxides
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- National Science Foundation
- U.S. Department of Energy
- Gordon and Betty Moore Foundation
- Division of Materials Research
- Basic Energy Sciences