An argument why the spinterface model cannot explain the chirality induced spin selectivity effect
In the context of chirality induced spin selectivity effect, it has been argued that a chiral molecule when adsorbed on a metal facilitates the formation of a local spin moment at the interface between the metal and molecule, given a strong spin-orbit coupling in the metal. The possibility for such spin moment formation is analyzed in terms of general arguments and effective modeling of a pertinent setup. The conclusion from this analysis is that a strong spin-orbit coupling in the metal does not provide a sufficient mechanism to sustain a stabilized spin moment at the interface. It is, moreover, shown that an electron flux into or out of the molecule does not provide conditions for a spin moment formation, regardless of whether the flux is spin-polarized or not.
Authors
- Jonas Fransson (ORCID: https://orcid.org/0000-0002-9217-2218)
Institutions
- Uppsala University (SE)
Publication Details
- Journal
- The Journal of Chemical Physics
- Published
- 2026-06-09
- DOI
- https://doi.org/10.1063/5.0337054
- Primary Topic
- Molecular Junctions and Nanostructures
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Stiftelsen Olle Engkvist Byggmästare