PbSe/WTe <sub>2</sub> Schottky Heterojunction for Low-Noise Mid-Infrared Detection

Room-temperature midwave infrared (MWIR) detection is crucial for applications such as gas sensing, thermal imaging, and optical communications. However, conventional narrow-band gap semiconductors (such as HgCdTe, InAsSb, and PbSe) suffer from high dark current, leading to significant noise at room temperature. To address this challenge, we propose a hybrid-dimensional PbSe/WTe2 van der Waals heterostructure. The formed Schottky barrier effectively modulates carrier transport through the built-in electric field, resulting in significantly suppressed dark current density (as low as 6.9 × 10–5 A·cm–2) and noise current (8.3 × 10–13 A Hz–1/2). The dark current is reduced by approximately 1 order of magnitude compared to that of pure PbSe devices. Further, the device demonstrates a broad spectral response range from 808 to 4000 nm, with a peak responsivity of 0.75 A/W and specific detectivity of 4.81 × 109 cm Hz1/2 W–1 at 2600 nm, which are comparable with commercial MWIR detectors. Finally, we demonstrate a room-temperature clear blackbody and thermal target imaging by PbSe/WTe2 heterojunction, providing an effective pathway for low-noise room-temperature MWIR detectors.

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Publication Details

Journal
ACS Applied Materials & Interfaces
Published
2026-05-30
DOI
https://doi.org/10.1021/acsami.6c06229
Primary Topic
2D Materials and Applications
Type
article
Field-Weighted Citation Impact
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article

PbSe/WTe 2 Schottky Heterojunction for Low-Noise Mid-Infrared Detection

Fafu Liu, Mingshuo Zhen, Q Wang, Fengliang Liu et al.
ACS Applied Materials & Interfaces
2D Materials and Applications
article

PbSe/WTe 2 Schottky Heterojunction for Low-Noise Mid-Infrared Detection

Fafu Liu, Mingshuo Zhen, Q Wang, Fengliang Liu, Xi Zhang, Xiangting Wang, Shengpeng Yuan, Yu Wan
article en

Abstract

Room-temperature midwave infrared (MWIR) detection is crucial for applications such as gas sensing, thermal imaging, and optical communications. However, conventional narrow-band gap semiconductors (such as HgCdTe, InAsSb, and PbSe) suffer from high dark current, leading to significant noise at room temperature. To address this challenge, we propose a hybrid-dimensional PbSe/WTe2 van der Waals heterostructure. The formed Schottky barrier effectively modulates carrier transport through the built-in electric field, resulting in significantly suppressed dark current density (as low as 6.9 × 10–5 A·cm–2) and noise current (8.3 × 10–13 A Hz–1/2). The dark current is reduced by approximately 1 order of magnitude compared to that of pure PbSe devices. Further, the device demonstrates a broad spectral response range from 808 to 4000 nm, with a peak responsivity of 0.75 A/W and specific detectivity of 4.81 × 109 cm Hz1/2 W–1 at 2600 nm, which are comparable with commercial MWIR detectors. Finally, we demonstrate a room-temperature clear blackbody and thermal target imaging by PbSe/WTe2 heterojunction, providing an effective pathway for low-noise room-temperature MWIR detectors.

ACS Applied Materials & Interfaces
Jiangnan University (CN), Nanchang University (CN), Department of Physics, Mathematics and Informatics (BY), Division of Materials Science and Engineering (AU)
Natural Science Foundation of Jiangxi Province
Affordable and clean energy
Openalex Percentile: Top 12%
2D Materials and Applications
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