Linear magneto-birefringence as a probe of altermagnetism

Altermagnets are a class of magnets that exhibit non-relativistic spin splitting (NRSS) of electronic bands in the absence of net magnetization. Their potential to generate large spin polarization without spin-orbit coupling has created strong interest in probes that access the underlying order parameter directly. In this Perspective, we show that linear magneto-birefringence (LMB) provides a natural and broadly applicable route to detecting altermagnetic order. Building on the correspondence between the momentum-space structure of NRSS and the ferroic ordering of magnetic multipoles in real space, we demonstrate how d-wave and g-wave NRSS textures yield distinct LMB responses. We present a symmetry-based framework that identifies the optical geometries and field configurations required to isolate specific multipole components, enabling domain imaging and providing benchmarks for theoretical models of LMB.

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Publication Details

Journal
npj Quantum Materials
Published
2026-05-30
DOI
https://doi.org/10.1038/s41535-026-00901-8
Primary Topic
Magnetic properties of thin films
Type
article
Field-Weighted Citation Impact
0.00

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article

Linear magneto-birefringence as a probe of altermagnetism

V. Sunko, J. Orenstein
npj Quantum Materials
Magnetic properties of thin films
article

Linear magneto-birefringence as a probe of altermagnetism

V. Sunko, J. Orenstein
article en

Abstract

Altermagnets are a class of magnets that exhibit non-relativistic spin splitting (NRSS) of electronic bands in the absence of net magnetization. Their potential to generate large spin polarization without spin-orbit coupling has created strong interest in probes that access the underlying order parameter directly. In this Perspective, we show that linear magneto-birefringence (LMB) provides a natural and broadly applicable route to detecting altermagnetic order. Building on the correspondence between the momentum-space structure of NRSS and the ferroic ordering of magnetic multipoles in real space, we demonstrate how d-wave and g-wave NRSS textures yield distinct LMB responses. We present a symmetry-based framework that identifies the optical geometries and field configurations required to isolate specific multipole components, enabling domain imaging and providing benchmarks for theoretical models of LMB.

npj Quantum Materials
Institute of Science and Technology Austria (AT), University of California, Berkeley (US)
Gordon and Betty Moore Foundation
Openalex Percentile: Top 5%
Magnetic properties of thin films
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