Photoacoustic Multigas Sensor via CNN-Based Mode Division Multiplexing

Photoacoustic multigas detection has important applications in fields such as environmental monitoring and fault diagnosis of power equipment. However, existing detection technologies all have inherent limitations: time division multiplexing (TDM) cannot realize simultaneous multigas detection; frequency division multiplexing (FDM) faces challenges such as complex frequency resource allocation and increased system costs; mode division multiplexing (MDM) technology enables simultaneous same-frequency detection, but it relies on a restrictive assumption that different gas signals exhibit distinct waveform widths and are linearly superimposed, which limits its universality. This paper proposes a convolutional neural network-based mode division multiplexing (CNN-MDM) technology. This technology is not only applicable to various different waveform characteristics, but is also capable of accommodating both linear and nonlinear superposition scenarios, thereby providing a universal MDM solution. The core of this scheme lies in assigning unique waveform characteristics to different gases at the modulation stage, and then identifying and separating the mixed signals through a CNN. Experiments were conducted using the decomposition components of SF6, namely H2S and CO, as the detection targets. The results demonstrate that the signals separated by the neural network exhibit a strong linear relationship with gas concentrations, with linear fit R2 values of 0.996 and 0.995 for CO and H2S, respectively, and detection limits of 50 and 426 ppb. This CNN-MDM scheme provides a universal framework for simultaneous same-frequency multigas detection and can be extended to photoacoustic systems with mixed modulation modes as well as tunable diode laser absorption spectroscopy (TDLAS).

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Publication Details

Journal
Analytical Chemistry
Published
2026-05-27
DOI
https://doi.org/10.1021/acs.analchem.6c02180
Primary Topic
Spectroscopy and Laser Applications
Type
article
Field-Weighted Citation Impact
0.00

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article

Photoacoustic Multigas Sensor via CNN-Based Mode Division Multiplexing

X.C. Li, 牧凯军, Qi Wang, Li Li et al.
Analytical Chemistry
Spectroscopy and Laser Applications
article

Photoacoustic Multigas Sensor via CNN-Based Mode Division Multiplexing

X.C. Li, 牧凯军, Qi Wang, Li Li, Pengbo Chen, Chongxin Shan, YingYing Qiao, Mingyang Feng, Mu Liang, Mingqi Jiao
article en

Abstract

Photoacoustic multigas detection has important applications in fields such as environmental monitoring and fault diagnosis of power equipment. However, existing detection technologies all have inherent limitations: time division multiplexing (TDM) cannot realize simultaneous multigas detection; frequency division multiplexing (FDM) faces challenges such as complex frequency resource allocation and increased system costs; mode division multiplexing (MDM) technology enables simultaneous same-frequency detection, but it relies on a restrictive assumption that different gas signals exhibit distinct waveform widths and are linearly superimposed, which limits its universality. This paper proposes a convolutional neural network-based mode division multiplexing (CNN-MDM) technology. This technology is not only applicable to various different waveform characteristics, but is also capable of accommodating both linear and nonlinear superposition scenarios, thereby providing a universal MDM solution. The core of this scheme lies in assigning unique waveform characteristics to different gases at the modulation stage, and then identifying and separating the mixed signals through a CNN. Experiments were conducted using the decomposition components of SF6, namely H2S and CO, as the detection targets. The results demonstrate that the signals separated by the neural network exhibit a strong linear relationship with gas concentrations, with linear fit R2 values of 0.996 and 0.995 for CO and H2S, respectively, and detection limits of 50 and 426 ppb. This CNN-MDM scheme provides a universal framework for simultaneous same-frequency multigas detection and can be extended to photoacoustic systems with mixed modulation modes as well as tunable diode laser absorption spectroscopy (TDLAS).

Analytical Chemistry
Zhongyuan University of Technology (CN), Zhengzhou University (CN), Ministry of Education (BD)
National Natural Science Foundation of China, National Key Scientific Instrument and Equipment Development Projects of China
Openalex Percentile: Top 11%
Spectroscopy and Laser Applications
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