Emergent Spin Supersolids in Frustrated Quantum Materials

Recent years have witnessed the emergence of spin supersolids in frustrated quantum magnets, establishing a material-based platform for supersolidity beyond its original context in solid helium. A spin supersolid is characterized by the coexistence of longitudinal spin order that breaks lattice translational symmetry and transverse spin order associated with the spontaneous breaking of the spin U(1) symmetry. Extensive experimental investigations, together with advanced numerical studies, have now revealed a coherent and internally consistent picture of these phases, substantially deepening our understanding of supersolidity in quantum magnetic materials. Beyond their fundamental interest as exotic quantum states, potential applications in highly efficient demagnetization cooling have been supported by a giant magnetocaloric effect observed in candidate materials. Moreover, the possible dissipationless spin supercurrents could open promising perspectives for spin transport and spintronic applications. This review summarizes recent progress on emergent spin supersolids in frustrated triangular-lattice quantum antiferromagnets, surveys experimental evidence from thermodynamic and spectroscopic measurements, and compares these results with theoretical studies of minimal models addressing global phase diagrams, ground state properties, and collective excitations. In addition, this review discusses characteristic spin-transport phenomena and outlines future directions for exploring spin supersolids as functional quantum materials.

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Publication Details

Journal
Advanced Materials
Published
2026-05-23
DOI
https://doi.org/10.1002/adma.202600005
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
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article

Emergent Spin Supersolids in Frustrated Quantum Materials

Seiji Yunoki, Yixuan Huang, Sadamichi Maekawa
Advanced Materials
Advanced Condensed Matter Physics
article

Emergent Spin Supersolids in Frustrated Quantum Materials

Seiji Yunoki, Yixuan Huang, Sadamichi Maekawa
article en

Abstract

Recent years have witnessed the emergence of spin supersolids in frustrated quantum magnets, establishing a material-based platform for supersolidity beyond its original context in solid helium. A spin supersolid is characterized by the coexistence of longitudinal spin order that breaks lattice translational symmetry and transverse spin order associated with the spontaneous breaking of the spin U(1) symmetry. Extensive experimental investigations, together with advanced numerical studies, have now revealed a coherent and internally consistent picture of these phases, substantially deepening our understanding of supersolidity in quantum magnetic materials. Beyond their fundamental interest as exotic quantum states, potential applications in highly efficient demagnetization cooling have been supported by a giant magnetocaloric effect observed in candidate materials. Moreover, the possible dissipationless spin supercurrents could open promising perspectives for spin transport and spintronic applications. This review summarizes recent progress on emergent spin supersolids in frustrated triangular-lattice quantum antiferromagnets, surveys experimental evidence from thermodynamic and spectroscopic measurements, and compares these results with theoretical studies of minimal models addressing global phase diagrams, ground state properties, and collective excitations. In addition, this review discusses characteristic spin-transport phenomena and outlines future directions for exploring spin supersolids as functional quantum materials.

Advanced Materials
Japan Atomic Energy Agency (JP), Pioneer (United States) (US), RIKEN (JP), RIKEN Center for Computational Science (JP), RIKEN Center for Emergent Matter Science (JP), RIKEN Center for Advanced Photonics (JP)
Openalex Percentile: Top 6%
Advanced Condensed Matter Physics
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