Optically Modulated Waveguide-Coupled Spintronic Terahertz Radiation Emitters

Terahertz (THz) waves have garnered growing attention for applications in communication, imaging, and spectroscopy, yet compact and efficient on-chip THz sources remain scarce. In this work, we achieve the in-situ generation, modulation, and sensing of coherent THz radiation within a single chip-scale device. We fabricate a waveguide-fed spintronic THz emitter comprising a silicon dioxide layer sandwiched between two W/Fe/Pt multilayers, integrating THz emission and modulation functionalities into a monolithic platform. Magnetic-field and symmetry-dependent measurements under both normal and side illumination confirm that the emitted broadband THz radiation originates from spin-to-charge conversion in the W/Fe/Pt multilayer structure. We further demonstrate that, under side excitation, the amplitude of the THz signal can be efficiently controlled by varying the pump polarization, enabling all-optical in-situ modulation without any external components. Numerical simulations elucidate the physical mechanism underlying this polarization-dependent modulation. Finally, we employ the device to measure the characteristic spectral response of α-lactose, validating its potential for on-chip spectroscopic sensing. This work offers a compact and integrable strategy for the simultaneous generation and manipulation of THz waves, paving a promising route toward chip-scale THz communication, imaging, and sensing systems.

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Publication Details

Journal
The Journal of Physical Chemistry Letters
Published
2026-05-22
DOI
https://doi.org/10.1021/acs.jpclett.6c01322
Primary Topic
Magnetic properties of thin films
Type
article
Field-Weighted Citation Impact
0.00

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article

Optically Modulated Waveguide-Coupled Spintronic Terahertz Radiation Emitters

Z Li, Chen Huang, Bo Lu, Zhenjie Ge et al.
The Journal of Physical Chemistry Letters
Magnetic properties of thin films
article

Optically Modulated Waveguide-Coupled Spintronic Terahertz Radiation Emitters

Z Li, Chen Huang, Bo Lu, Zhenjie Ge, Zuanming Jin, Xianyang Lu, Yongbing Xu, Zhiqiang Lan
article en

Abstract

Terahertz (THz) waves have garnered growing attention for applications in communication, imaging, and spectroscopy, yet compact and efficient on-chip THz sources remain scarce. In this work, we achieve the in-situ generation, modulation, and sensing of coherent THz radiation within a single chip-scale device. We fabricate a waveguide-fed spintronic THz emitter comprising a silicon dioxide layer sandwiched between two W/Fe/Pt multilayers, integrating THz emission and modulation functionalities into a monolithic platform. Magnetic-field and symmetry-dependent measurements under both normal and side illumination confirm that the emitted broadband THz radiation originates from spin-to-charge conversion in the W/Fe/Pt multilayer structure. We further demonstrate that, under side excitation, the amplitude of the THz signal can be efficiently controlled by varying the pump polarization, enabling all-optical in-situ modulation without any external components. Numerical simulations elucidate the physical mechanism underlying this polarization-dependent modulation. Finally, we employ the device to measure the characteristic spectral response of α-lactose, validating its potential for on-chip spectroscopic sensing. This work offers a compact and integrable strategy for the simultaneous generation and manipulation of THz waves, paving a promising route toward chip-scale THz communication, imaging, and sensing systems.

The Journal of Physical Chemistry Letters
Tongji University (CN), University of Shanghai for Science and Technology (CN), Shenzhen Terahertz Technology Innovation Research Institute (CN), Photonic Science (United Kingdom) (GB), Spintronics Research Network of Japan (JP), Nanjing University (CN)
National Natural Science Foundation of China, Shanghai Educational Development Foundation, Science and Technology Commission of Shanghai Municipality, Natural Science Foundation of Jiangsu Province, Higher Education Discipline Innovation Project, General Administration of Customs, National Key Research and Development Program of China
Affordable and clean energy
Openalex Percentile: Top 6%
Magnetic properties of thin films
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