Nodeless superconducting gap and electron-boson coupling in (La,Pr,Sm) <sub>3</sub> Ni <sub>2</sub> O <sub>7</sub> films

The discovery of superconductivity in Ruddlesden-Popper (RP) bilayer nickelate films under ambient pressure provides an opportunity to directly investigate electronic energy scales of the superconducting state and the pairing mechanism. We report angle-resolved photoemission spectroscopy measurements of superconducting (La,Pr,Sm) 3 Ni 2 O 7 thin films by developing an ultra-high vacuum cryogenic sample quenching and transfer technique. A superconducting gap of ~18 meV with coherence peaks is observed along the Brillouin zone diagonal. The finite gap persists across the entire Brillouin zone, revealing the absence of gap nodes. A kink is observed in the energy-momentum dispersion at ~70 meV below Fermi level, indicating an electron-boson coupling. The simultaneous observation of a nodeless superconducting gap and electron-boson coupling provides insight into the pairing symmetry and gluing mechanism in RP bilayer nickelates.

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Journal
Science
Published
2026-05-21
DOI
https://doi.org/10.1126/science.adw8329
Primary Topic
Magnetic and transport properties of perovskites and related materials
Type
article
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article

Nodeless superconducting gap and electron-boson coupling in (La,Pr,Sm) 3 Ni 2 O 7 films

Lizhi Xu, Y Li, Yaqi Chen, Jianchang Shen et al.
Science
Magnetic and transport properties of perovskites and related materials
article

Nodeless superconducting gap and electron-boson coupling in (La,Pr,Sm) 3 Ni 2 O 7 films

Lizhi Xu, Y Li, Yaqi Chen, Jianchang Shen, Peng Li, Zihao Nie, Guangdi Zhou, Han Sun, Junfeng He, H Wang, Zechao Wang, Runqing Luan, Yu Miao, Haoliang Huang, Zhuoyu Chen, Zhipeng Ou, Wei Lv, Xinru Yong, Zikun Feng, Yu-Jie Sun, Qi-Kun Xue
article en

Abstract

The discovery of superconductivity in Ruddlesden-Popper (RP) bilayer nickelate films under ambient pressure provides an opportunity to directly investigate electronic energy scales of the superconducting state and the pairing mechanism. We report angle-resolved photoemission spectroscopy measurements of superconducting (La,Pr,Sm) 3 Ni 2 O 7 thin films by developing an ultra-high vacuum cryogenic sample quenching and transfer technique. A superconducting gap of ~18 meV with coherence peaks is observed along the Brillouin zone diagonal. The finite gap persists across the entire Brillouin zone, revealing the absence of gap nodes. A kink is observed in the energy-momentum dispersion at ~70 meV below Fermi level, indicating an electron-boson coupling. The simultaneous observation of a nodeless superconducting gap and electron-boson coupling provides insight into the pairing symmetry and gluing mechanism in RP bilayer nickelates.

Science
University of Science and Technology of China (CN), Southern University of Science and Technology (CN), Hefei National Center for Physical Sciences at Nanoscale (CN), Quantum Science Center of Guangdong-Hong Kong-Macao Greater Bay Area (CN), Tsinghua University (CN)
Affordable and clean energy
Openalex Percentile: Top 14%
Magnetic and transport properties of perovskites and related materials
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