Vortex order in magnetic frustrated GeNi2O4 and GeCo2O4 spinels

In the search for new spin textures based on singular magnetic objects like Bloch-points or vortices, spinel compounds emerge as an interesting playground due to the interplay between magnetic anisotropy and complex interactions that extend well beyond first neighbors on a pyrochlore lattice. Based on an exploration of the exchange interaction phase diagrams of members of the Ge$B_2$O$_4$ family with $B$=Co and Ni, we show, using simultaneous modeling of inelastic neutron scattering measurements and single-crystal neutron diffraction data, that a 2-$k$ magnetic structure may be stabilized in these compounds. This leads to a short period spin vortex crystal, a variant induced by the magnetic anisotropy of the 3-$k$ Bloch-point structure predicted for isotropic spins. Our study rationalizes the formation of these multi-$k$ spin textures in frustrated antiferromagnets, as well as their anisotropy-dependent evolution.

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Publication Details

Journal
Physical Review Research
Published
2026-11-04
DOI
https://doi.org/10.1103/ywbl-flp1
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
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article

Vortex order in magnetic frustrated GeNi2O4 and GeCo2O4 spinels

J. Ollivier, M. Songvilay, N. Qureshi, B. Fåk et al.
Physical Review Research
Advanced Condensed Matter Physics
article

Vortex order in magnetic frustrated GeNi2O4 and GeCo2O4 spinels

J. Ollivier, M. Songvilay, N. Qureshi, B. Fåk, E. Ressouche, Pierre Strobel, J. Robert, S. Petit, V. Simonet, K. Beauvois, S. Lenne, P. Manuel, S. DeBrion, R. Ballou
article en

Abstract

In the search for new spin textures based on singular magnetic objects like Bloch-points or vortices, spinel compounds emerge as an interesting playground due to the interplay between magnetic anisotropy and complex interactions that extend well beyond first neighbors on a pyrochlore lattice. Based on an exploration of the exchange interaction phase diagrams of members of the Ge$B_2$O$_4$ family with $B$=Co and Ni, we show, using simultaneous modeling of inelastic neutron scattering measurements and single-crystal neutron diffraction data, that a 2-$k$ magnetic structure may be stabilized in these compounds. This leads to a short period spin vortex crystal, a variant induced by the magnetic anisotropy of the 3-$k$ Bloch-point structure predicted for isotropic spins. Our study rationalizes the formation of these multi-$k$ spin textures in frustrated antiferromagnets, as well as their anisotropy-dependent evolution.

Physical Review Research
Openalex Percentile: Top 71%
Advanced Condensed Matter Physics
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