Superconducting Cavity Probes Sliding Ferroelectricity in Small-Angle Twisted WSe <sub>2</sub>

Ferroelectricity is a property of materials that exhibits spontaneous charge polarization. Ferroelectricity in 2D materials is interesting because of its applications in memory devices and field-effect transistors. Recently, a new type of ferroelectricity, known as sliding ferroelectricity, has been discovered, in which parallel-stacked bilayers of hexagonal boron nitride (hBN) or transition metal dichalcogenides (TMDCs) develop an out-of-plane electric polarization. In this work, we probe the polarization of small-angle parallel-stacked WSe2 by measuring its high-frequency AC response, achieved by embedding it into a half-wave superconducting coplanar waveguide cavity. We observe a hysteretic response in the capacitance of the stack and the quality factor of the cavity, confirming ferroelectric switching in the system. Our results further reveal relaxation effects associated with the ferroelectric domain wall motion. This cavity-based technique has potential applications in probing domain wall dynamics in a ferroelectric system at high frequencies.

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Publication Details

Journal
Nano Letters
Published
2026-05-18
DOI
https://doi.org/10.1021/acs.nanolett.6c02041
Primary Topic
2D Materials and Applications
Type
article
Field-Weighted Citation Impact
0.00

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article

Superconducting Cavity Probes Sliding Ferroelectricity in Small-Angle Twisted WSe 2

Supriya Mandal, Meghan P. Patankar, Mandar M. Deshmukh, Vibhor Singh et al.
Nano Letters
2D Materials and Applications
article

Superconducting Cavity Probes Sliding Ferroelectricity in Small-Angle Twisted WSe 2

Supriya Mandal, Meghan P. Patankar, Mandar M. Deshmukh, Vibhor Singh, Krishnendu Maji, Rishiraj Rajkhowa, Sayani Pal, Malhar Date, Kenji Watanabe, Takashi Taniguchi, Sriram H.
article en

Abstract

Ferroelectricity is a property of materials that exhibits spontaneous charge polarization. Ferroelectricity in 2D materials is interesting because of its applications in memory devices and field-effect transistors. Recently, a new type of ferroelectricity, known as sliding ferroelectricity, has been discovered, in which parallel-stacked bilayers of hexagonal boron nitride (hBN) or transition metal dichalcogenides (TMDCs) develop an out-of-plane electric polarization. In this work, we probe the polarization of small-angle parallel-stacked WSe2 by measuring its high-frequency AC response, achieved by embedding it into a half-wave superconducting coplanar waveguide cavity. We observe a hysteretic response in the capacitance of the stack and the quality factor of the cavity, confirming ferroelectric switching in the system. Our results further reveal relaxation effects associated with the ferroelectric domain wall motion. This cavity-based technique has potential applications in probing domain wall dynamics in a ferroelectric system at high frequencies.

Nano Letters
Tata Institute of Fundamental Research (IN), Centre National de la Recherche Scientifique (FR), National Institute for Materials Science (JP), Institut Néel (FR), Indian Institute of Science Bangalore (IN), Université Grenoble Alpes (FR)
Department of Science and Technology, Ministry of Science and Technology, India, Department of Atomic Energy, Government of India, Ministry of Education, Culture, Sports, Science and Technology, Japan Society for the Promotion of Science, Nano Mission Council, Air Force Office of Scientific Research
Affordable and clean energy
Openalex Percentile: Top 11%
2D Materials and Applications
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