Ultrafine Nanoporous Ordered High-Entropy Intermetallics with Isolated Multisites toward Electrocatalytic Aldehyde Hydrogenation
-(C, O)-aldehyde adsorption configuration for C═O bond activation and facilitate a highly interconnected two-coordinated hydrogen-bonded network for directional H* transfer and suppressing the competitive hydrogen evolution reaction (HER). The presented Zn-EPT strategy for synthesizing ultrafine np-HEIs offers a general blueprint for designing high-efficiency electrocatalysts for electrocatalytic hydrogenation and other related applications.
Authors
- Fang Wang (ORCID: https://orcid.org/0000-0002-5971-2622)
- J W Li
- Chengjin Dong
- Zhen Wang
- Jiao Lan
- Jiuhui Han (ORCID: https://orcid.org/0000-0002-9067-9197)
- Linghu Meng
- Yongwen Tan (ORCID: https://orcid.org/0000-0003-1486-4048)
Institutions
- Tianjin University of Technology (CN)
- Hunan University (CN)
- Division of Materials Science and Engineering (AU)
Publication Details
- Journal
- Journal of the American Chemical Society
- Published
- 2026-05-08
- DOI
- https://doi.org/10.1021/jacs.6c02792
- Primary Topic
- Electrocatalysts for Energy Conversion
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- National Natural Science Foundation of China
- State Key Laboratory of Advanced Design and Manufacturing for Vehicle Body