Spectrum Shaping of the Ultrabroadband Terahertz Radiation from Air Plasma Driven by Two-Color Bifilamentation

We report on the generation and spectral shaping of ultrabroadband terahertz-to-infrared radiation (>119 THz) from air plasma excited by a conventional tightly focused femtosecond Ti:Sa laser pulse with a duration of 35 fs assisted by its second harmonic (SH). A controllable and large frequency detuning between the SH and blueshifted component of the fundamental spectrum was achieved by utilizing spectral broadening of the fundamental pulse under filamentation and adjusting the longitudinal separation of the two cascaded filaments. For convenience, the resulting ultrabroadband emission is divided into a low-frequency part (<30 THz), an intermediate-frequency part (~50 THz), and a high-frequency part (~100 THz) that can be optimized with the filaments’ longitudinal separation. We attribute such ultrabroadband THz radiation generation to the excitation of photocurrent from the nonlinear interaction of SH with both the field at the fundamental frequency and its blueshifted component acquired during filamentation. Theoretical calculations based on time-dependent Schrödinger equation, as well as the Maxwell–Schrödinger equation for spectral broadening dynamics, reproduced the spectral features as well as the distinct dependence of the low- and high-frequency THz components.