Process intensification of solid‐sorbent <scp>DAC</scp> via a rotating vortex reactor

Abstract This work investigates the performance of the rotating vortex reactor (RVR) as a promising intensified contactor for direct air capture (DAC). Both adsorption and desorption are tested across ranges of superficial gas velocities and rotation speeds, thereby tuning the bed regime—packed or fluidized—under a centrifugal force field (known as a high‐gravity condition) and a vortex flow to enhance mass and heat transfer. A cyclic cut‐off analysis further quantifies the contributions of the main energy consumers and clarifies the trade‐offs between productivity and energy demand. The adsorber achieves high volumetric CO 2 capture rates of 7.5–13.5 kgCO 2 /(m 3 ·h), while hot‐air regeneration enables rapid desorption in &lt;10 min. This proof‐of‐concept study shows RVR's potential for process intensification while identifying areas for further improvement in the unit's design and operation to reduce energy demand for DAC.

Authors

Institutions

Publication Details

Journal
AIChE Journal
Published
2026-04-29
DOI
https://doi.org/10.1002/aic.70421
Primary Topic
Carbon Dioxide Capture Technologies
Type
article
Field-Weighted Citation Impact
0.00

Funders

Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Process intensification of solid‐sorbent DAC via a rotating vortex reactor

Geraldine J. Heynderickx, Afroditi Kourou, Siyuan Chen, Bing Wang et al.
AIChE Journal
Carbon Dioxide Capture Technologies
article

Process intensification of solid‐sorbent DAC via a rotating vortex reactor

Geraldine J. Heynderickx, Afroditi Kourou, Siyuan Chen, Bing Wang, Yi Ouyang, Kevin M. Van Geem
article en

Abstract

Abstract This work investigates the performance of the rotating vortex reactor (RVR) as a promising intensified contactor for direct air capture (DAC). Both adsorption and desorption are tested across ranges of superficial gas velocities and rotation speeds, thereby tuning the bed regime—packed or fluidized—under a centrifugal force field (known as a high‐gravity condition) and a vortex flow to enhance mass and heat transfer. A cyclic cut‐off analysis further quantifies the contributions of the main energy consumers and clarifies the trade‐offs between productivity and energy demand. The adsorber achieves high volumetric CO 2 capture rates of 7.5–13.5 kgCO 2 /(m 3 ·h), while hot‐air regeneration enables rapid desorption in &lt;10 min. This proof‐of‐concept study shows RVR's potential for process intensification while identifying areas for further improvement in the unit's design and operation to reduce energy demand for DAC.

AIChE Journal
Ghent University (BE)
Agentschap Innoveren en Ondernemen, Fonds Wetenschappelijk Onderzoek, Fondation Francqui - Stichting, HORIZON EUROPE European Research Council
Affordable and clean energy
Openalex Percentile: Top 11%
Carbon Dioxide Capture Technologies
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.

Process intensification of solid‐sorbent <scp>DAC</scp> via a rotating vortex reactor — Geraldine J. Heynderickx, Afroditi Kourou, et al. · AIChE Journal (2026) | TGRS Research Map | TGRS