Process intensification of solid‐sorbent <scp>DAC</scp> via a rotating vortex reactor
Abstract This work investigates the performance of the rotating vortex reactor (RVR) as a promising intensified contactor for direct air capture (DAC). Both adsorption and desorption are tested across ranges of superficial gas velocities and rotation speeds, thereby tuning the bed regime—packed or fluidized—under a centrifugal force field (known as a high‐gravity condition) and a vortex flow to enhance mass and heat transfer. A cyclic cut‐off analysis further quantifies the contributions of the main energy consumers and clarifies the trade‐offs between productivity and energy demand. The adsorber achieves high volumetric CO 2 capture rates of 7.5–13.5 kgCO 2 /(m 3 ·h), while hot‐air regeneration enables rapid desorption in <10 min. This proof‐of‐concept study shows RVR's potential for process intensification while identifying areas for further improvement in the unit's design and operation to reduce energy demand for DAC.
Authors
- Geraldine J. Heynderickx (ORCID: https://orcid.org/0000-0002-0713-9588)
- Afroditi Kourou (ORCID: https://orcid.org/0000-0002-1059-2367)
- Siyuan Chen (ORCID: https://orcid.org/0000-0002-4530-9576)
- Bing Wang (ORCID: https://orcid.org/0009-0003-9246-2316)
- Yi Ouyang (ORCID: https://orcid.org/0000-0002-1950-4538)
- Kevin M. Van Geem (ORCID: https://orcid.org/0000-0003-4191-4960)
Institutions
- Ghent University (BE)
Publication Details
- Journal
- AIChE Journal
- Published
- 2026-04-29
- DOI
- https://doi.org/10.1002/aic.70421
- Primary Topic
- Carbon Dioxide Capture Technologies
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Agentschap Innoveren en Ondernemen
- Fonds Wetenschappelijk Onderzoek
- Fondation Francqui - Stichting
- HORIZON EUROPE European Research Council