Microscopic study of thermally and electrically driven magnetic changes in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi mathvariant="normal">La</mml:mi> <mml:mrow> <mml:mn>0.7</mml:mn> </mml:mrow> </mml:msub

Epitaxial films of the ferromagnetic manganite <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:mrow> <a:msub> <a:mi mathvariant="normal">La</a:mi> <a:mrow> <a:mn>0.7</a:mn> </a:mrow> </a:msub> <a:msub> <a:mi mathvariant="normal">Sr</a:mi> <a:mrow> <a:mn>0.3</a:mn> </a:mrow> </a:msub> <a:msub> <a:mi>MnO</a:mi> <a:mn>3</a:mn> </a:msub> </a:mrow> </a:math> on substrates of the ferroelectric perovskite <d:math xmlns:d="http://www.w3.org/1998/Math/MathML"> <d:mrow> <d:msub> <d:mi>BaTiO</d:mi> <d:mn>3</d:mn> </d:msub> </d:mrow> </d:math> are known to display sharp magnetic changes and large magnetoelectric effects when the film is strained by the substrate undergoing thermally driven structural transitions and ferroelectric domain switching, respectively. However, only a single component of the in-plane magnetization has been hitherto imaged. Here we present magnetic vector maps—obtained from photoemission electron microscopy images with magnetic contrast from x-ray magnetic circular dichroism—to show that the electrically and thermally driven changes of local and global magnetization are deterministically influenced by the state of the substrate while also being complex and sample dependent. Our findings, supported by ferromagnetic resonance data and vibrating sample magnetometry, reveal that the behavior of <e:math xmlns:e="http://www.w3.org/1998/Math/MathML"> <e:mrow> <e:msub> <e:mi mathvariant="normal">La</e:mi> <e:mrow> <e:mn>0.7</e:mn> </e:mrow> </e:msub> <e:msub> <e:mi mathvariant="normal">Sr</e:mi> <e:mrow> <e:mn>0.3</e:mn> </e:mrow> </e:msub> <e:msub> <e:mi>MnO</e:mi> <e:mn>3</e:mn> </e:msub> </e:mrow> </e:math> films on <h:math xmlns:h="http://www.w3.org/1998/Math/MathML"> <h:mrow> <h:msub> <h:mi>BaTiO</h:mi> <h:mn>3</h:mn> </h:msub> </h:mrow> </h:math> substrates is not well predicted from knowledge of each system, probably due to long-range strain between <i:math xmlns:i="http://www.w3.org/1998/Math/MathML"> <i:mrow> <i:msub> <i:mi>BaTiO</i:mi> <i:mn>3</i:mn> </i:msub> </i:mrow> </i:math> domains. In the future, it would be interesting to reduce complexity by patterning the film into regions between which magnetic communication is negligible.

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Publication Details

Journal
Physical Review Materials
Published
2026-05-01
DOI
https://doi.org/10.1103/rgyl-7zk5
Primary Topic
Multiferroics and related materials
Type
article
Field-Weighted Citation Impact
0.00

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article

Microscopic study of thermally and electrically driven magnetic changes in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi mathvariant="normal">La</mml:mi> <mml:mrow> <mml:mn>0.7</mml:mn> </mml:mrow> </mml:msub

F. Maccherozzi, Т. И. Полек, А. И. Товстолыткин, S. S. Dhesi et al.
Physical Review Materials
Multiferroics and related materials
article

Microscopic study of thermally and electrically driven magnetic changes in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi mathvariant="normal">La</mml:mi> <mml:mrow> <mml:mn>0.7</mml:mn> </mml:mrow> </mml:msub

F. Maccherozzi, Т. И. Полек, А. И. Товстолыткин, S. S. Dhesi, M. Ghidini, X. Moya, L. C. Phillips, N. D. Mathur, D. M. Polishchuk
article en

Abstract

Epitaxial films of the ferromagnetic manganite <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:mrow> <a:msub> <a:mi mathvariant="normal">La</a:mi> <a:mrow> <a:mn>0.7</a:mn> </a:mrow> </a:msub> <a:msub> <a:mi mathvariant="normal">Sr</a:mi> <a:mrow> <a:mn>0.3</a:mn> </a:mrow> </a:msub> <a:msub> <a:mi>MnO</a:mi> <a:mn>3</a:mn> </a:msub> </a:mrow> </a:math> on substrates of the ferroelectric perovskite <d:math xmlns:d="http://www.w3.org/1998/Math/MathML"> <d:mrow> <d:msub> <d:mi>BaTiO</d:mi> <d:mn>3</d:mn> </d:msub> </d:mrow> </d:math> are known to display sharp magnetic changes and large magnetoelectric effects when the film is strained by the substrate undergoing thermally driven structural transitions and ferroelectric domain switching, respectively. However, only a single component of the in-plane magnetization has been hitherto imaged. Here we present magnetic vector maps—obtained from photoemission electron microscopy images with magnetic contrast from x-ray magnetic circular dichroism—to show that the electrically and thermally driven changes of local and global magnetization are deterministically influenced by the state of the substrate while also being complex and sample dependent. Our findings, supported by ferromagnetic resonance data and vibrating sample magnetometry, reveal that the behavior of <e:math xmlns:e="http://www.w3.org/1998/Math/MathML"> <e:mrow> <e:msub> <e:mi mathvariant="normal">La</e:mi> <e:mrow> <e:mn>0.7</e:mn> </e:mrow> </e:msub> <e:msub> <e:mi mathvariant="normal">Sr</e:mi> <e:mrow> <e:mn>0.3</e:mn> </e:mrow> </e:msub> <e:msub> <e:mi>MnO</e:mi> <e:mn>3</e:mn> </e:msub> </e:mrow> </e:math> films on <h:math xmlns:h="http://www.w3.org/1998/Math/MathML"> <h:mrow> <h:msub> <h:mi>BaTiO</h:mi> <h:mn>3</h:mn> </h:msub> </h:mrow> </h:math> substrates is not well predicted from knowledge of each system, probably due to long-range strain between <i:math xmlns:i="http://www.w3.org/1998/Math/MathML"> <i:mrow> <i:msub> <i:mi>BaTiO</i:mi> <i:mn>3</i:mn> </i:msub> </i:mrow> </i:math> domains. In the future, it would be interesting to reduce complexity by patterning the film into regions between which magnetic communication is negligible.

Physical Review MaterialsVol. 10(5)
University of Parma (IT), University of Cambridge (GB), Diamond Light Source (GB), Institute of Magnetism (UA)
Diamond Light Source, Royal Society, University of Cambridge, Departament d'Innovació, Universitats i Empresa, Generalitat de Catalunya, Ministero dell'Università e della Ricerca, National Academy of Sciences, Engineering and Physical Sciences Research Council, European Research Council
Openalex Percentile: Top 15%
Multiferroics and related materials
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