Asymmetric Fe–Te Pairs Enhance Peroxymonosulfate Activation via Surface‐Bound Hydroxyl Radicals Pathways
) plays a secondary role. As a result, FeTe DAs/NC achieves complete degradation of carbamazepine within 60 min, markedly outperforming Fe or Te single-atom analogs, together with excellent reactivity and cycling stability across different water matrices and pollutant systems. This work establishes atomic-scale asymmetry and metal-metalloid p-d coupling as an effective strategy for steering PMS activation chemistry toward long-lived interfacial radical states.
Authors
- Yuntong Sun (ORCID: https://orcid.org/0000-0001-8402-1770)
- Xuheng Li
- Tierui Zhang
- Sheng Wang
- Jong-Min Lee
- Min Zheng
- Chunli Wang
Institutions
- Xi'an University of Architecture and Technology (CN)
- Nanyang Technological University (SG)
- Daegu Gyeongbuk Institute of Science and Technology (KR)
- State Key Laboratory of Pollution Control and Resource Reuse (CN)
- Technical Institute of Physics and Chemistry (CN)
- The University of Adelaide (AU)
Publication Details
- Journal
- Angewandte Chemie International Edition
- Published
- 2026-05-02
- DOI
- https://doi.org/10.1002/anie.3343591
- Primary Topic
- Advanced oxidation water treatment
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- National Research Foundation of Korea