Superconductivity in bilayer La$_3$Ni$_2$O$_7$ : A review focusing on the strong-coupling Hund's rule assisted pairing mechanism

The discoveries of high-$T_c$ superconductivity (SC) in bulk bilayer La$_3$Ni$_2$O$_7$ under pressure and of ambient-pressure SC in compressively strained thin films provide an important platform for exploring unconventional SC. Experiments reveal orbital-dependent band renormalization and sizable interlayer magnetic correlations, and show that SC emerges in association with pressure- or strain-induced structural changes. However, the role of the $\\gamma$ band, the symmetyr of the superconducting gap, and the microscopic pairing mechanism remain unresolved. This article reviews the relevant experimental observations and theoretical developments, with a focus on the strong-coupling Hund-assisted interlayer-pairing scenario. Within this framework, the two active Ni $E_g$ orbitals play distinct roles. In the local strong-coupling limit, the nearly half-filled and heavily renormalized $3d_{z^2}$ orbitals experience a sizable antiferromagnetic exchange across the bilayer through the inner apical oxygen. This exchange is proposed to favor interlayer rung-singlet correlations and may produce an orbital-dependent pseudogap regime. The onsite Hund's coupling aligns the two $E_g$ spins and generates an effective interlayer exchange between the more itinerant $3d_{x^2-y^2}$ carriers. The resulting bilayer models favor an interlayer $s$-wave state and predict that electron doping strengthens pairing. The Hund-assisted scenario can accommodate either the presence or absence of a $\\gamma$ pocket, provided that the $3d_{z^2}$ sector retains substantial local-moment character and sizable interlayer spin correlations. We also compare this framework with weak- and intermediate-coupling theories and other strong-coupling proposals.

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Journal
Journal of Physics Condensed Matter
Published
2026-09-16
DOI
https://doi.org/10.1088/1361-648x/aea8b1
Primary Topic
Magnetic and transport properties of perovskites and related materials
Type
article
Field-Weighted Citation Impact
0.00

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article

Superconductivity in bilayer La$_3$Ni$_2$O$_7$ : A review focusing on the strong-coupling Hund's rule assisted pairing mechanism

Fan Yang, Congjun Wu, Chen Lu, Zhiming Pan
Journal of Physics Condensed Matter
Magnetic and transport properties of perovskites and related materials
article

Superconductivity in bilayer La$_3$Ni$_2$O$_7$ : A review focusing on the strong-coupling Hund's rule assisted pairing mechanism

Fan Yang, Congjun Wu, Chen Lu, Zhiming Pan
article en

Abstract

The discoveries of high-$T_c$ superconductivity (SC) in bulk bilayer La$_3$Ni$_2$O$_7$ under pressure and of ambient-pressure SC in compressively strained thin films provide an important platform for exploring unconventional SC. Experiments reveal orbital-dependent band renormalization and sizable interlayer magnetic correlations, and show that SC emerges in association with pressure- or strain-induced structural changes. However, the role of the $\gamma$ band, the symmetyr of the superconducting gap, and the microscopic pairing mechanism remain unresolved. This article reviews the relevant experimental observations and theoretical developments, with a focus on the strong-coupling Hund-assisted interlayer-pairing scenario. Within this framework, the two active Ni $E_g$ orbitals play distinct roles. In the local strong-coupling limit, the nearly half-filled and heavily renormalized $3d_{z^2}$ orbitals experience a sizable antiferromagnetic exchange across the bilayer through the inner apical oxygen. This exchange is proposed to favor interlayer rung-singlet correlations and may produce an orbital-dependent pseudogap regime. The onsite Hund's coupling aligns the two $E_g$ spins and generates an effective interlayer exchange between the more itinerant $3d_{x^2-y^2}$ carriers. The resulting bilayer models favor an interlayer $s$-wave state and predict that electron doping strengthens pairing. The Hund-assisted scenario can accommodate either the presence or absence of a $\gamma$ pocket, provided that the $3d_{z^2}$ sector retains substantial local-moment character and sizable interlayer spin correlations. We also compare this framework with weak- and intermediate-coupling theories and other strong-coupling proposals.

Journal of Physics Condensed Matter
Beijing Institute of Technology (CN), Hangzhou Normal University (CN), Xiamen University (CN), Westlake University (CN)
National Natural Science Foundation of China, Xiamen University
Openalex Percentile: Top 78%
Magnetic and transport properties of perovskites and related materials
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