Two-dimensional active polar semiflexible polymer under shear flow

The nonequilibrium structural and dynamical properties of semiflexible active polar polymers subject to linear flow are studied using numerical simulations. Filaments are confined in two dimensions and immersed in a fluid described by the Brownian multiparticle collision dynamics approach. The applied shear flow causes conformational changes in a polymer, aligns it along the flow direction, and induces a tumbling motion at high flow rates. In an intermediate, activity-dependent shear-rate regime, a characteristic scaling exponent for the mean-square end-to-end distance along the gradient direction is observed. This exponent appears to be determined by the semiflexibility of the polymer. The tumbling dynamics exhibits a characteristic time, with a stronger dependence on the Weissenberg number than that of flexible active or passive polymers. Activity strongly impacts the rheological properties of semiflexible polymers and even implies a negative viscosity for weak flows. At very large values of the shear rate, shear dominates over activity, and passive-polymer behavior is assumed.

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Publication Details

Journal
The Journal of Chemical Physics
Published
2026-04-22
DOI
https://doi.org/10.1063/5.0315709
Primary Topic
Micro and Nano Robotics
Type
article
Field-Weighted Citation Impact
0.00

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article

Two-dimensional active polar semiflexible polymer under shear flow

A. Lamura, Roland G. Winkler
The Journal of Chemical Physics
Micro and Nano Robotics
article

Two-dimensional active polar semiflexible polymer under shear flow

A. Lamura, Roland G. Winkler
article en

Abstract

The nonequilibrium structural and dynamical properties of semiflexible active polar polymers subject to linear flow are studied using numerical simulations. Filaments are confined in two dimensions and immersed in a fluid described by the Brownian multiparticle collision dynamics approach. The applied shear flow causes conformational changes in a polymer, aligns it along the flow direction, and induces a tumbling motion at high flow rates. In an intermediate, activity-dependent shear-rate regime, a characteristic scaling exponent for the mean-square end-to-end distance along the gradient direction is observed. This exponent appears to be determined by the semiflexibility of the polymer. The tumbling dynamics exhibits a characteristic time, with a stronger dependence on the Weissenberg number than that of flexible active or passive polymers. Activity strongly impacts the rheological properties of semiflexible polymers and even implies a negative viscosity for weak flows. At very large values of the shear rate, shear dominates over activity, and passive-polymer behavior is assumed.

The Journal of Chemical PhysicsVol. 164(16)
Forschungszentrum Jülich (DE), Istituto per le Applicazioni del Calcolo Mauro Picone (IT)
Ministero dell’Istruzione, dell’Università e della Ricerca
Openalex Percentile: Top 10%
Micro and Nano Robotics
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