Aging of droplet size distribution in stratocumulus clouds: regimes of droplet size distribution evolution

Abstract. The climatic impact of maritime stratocumulus clouds depends on the evolution of their droplet size distribution (DSD), yet the mechanisms controlling their variability during evaporation remain poorly constrained. Using large-eddy simulations coupled with a Lagrangian cloud model, we demonstrate that the DSD evolution follows two primary regimes: adiabatic growth and entrainment–descent. Within the latter, DSD evolution follows divergent pathways determined by the parcel's entrainment history: strong entrainment-driven dilution near the cloud top causes rapid broadening, whereas large-scale boundary-layer descent leads to gradual evaporation. Our Lagrangian analysis of the Damköhler number reveals that the commonly observed vertical transition from inhomogeneous to homogeneous mixing signatures does not necessarily reflect a change in the local mixing mechanism. Instead, it results from the vertical sorting of parcels with divergent histories. Parcels subject to strong entrainment retain inhomogeneous signatures throughout their descent, while those experiencing minimal dilution exhibit homogeneous-like characteristics regardless of altitude. This distinction helps resolve ambiguities in interpreting in situ observations where mixing history is often unknown. Finally, we propose a combined analytical–empirical formulation that captures the relative dispersion during both growth and evaporation.

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Publication Details

Journal
Atmospheric chemistry and physics
Published
2026-04-22
DOI
https://doi.org/10.5194/acp-26-5427-2026
Primary Topic
Atmospheric aerosols and clouds
Type
article
Field-Weighted Citation Impact
0.00

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article

Aging of droplet size distribution in stratocumulus clouds: regimes of droplet size distribution evolution

Fabian Hoffmann, Jung-Sub Lim
Atmospheric chemistry and physics
Atmospheric aerosols and clouds
article

Aging of droplet size distribution in stratocumulus clouds: regimes of droplet size distribution evolution

Fabian Hoffmann, Jung-Sub Lim
article en

Abstract

Abstract. The climatic impact of maritime stratocumulus clouds depends on the evolution of their droplet size distribution (DSD), yet the mechanisms controlling their variability during evaporation remain poorly constrained. Using large-eddy simulations coupled with a Lagrangian cloud model, we demonstrate that the DSD evolution follows two primary regimes: adiabatic growth and entrainment–descent. Within the latter, DSD evolution follows divergent pathways determined by the parcel's entrainment history: strong entrainment-driven dilution near the cloud top causes rapid broadening, whereas large-scale boundary-layer descent leads to gradual evaporation. Our Lagrangian analysis of the Damköhler number reveals that the commonly observed vertical transition from inhomogeneous to homogeneous mixing signatures does not necessarily reflect a change in the local mixing mechanism. Instead, it results from the vertical sorting of parcels with divergent histories. Parcels subject to strong entrainment retain inhomogeneous signatures throughout their descent, while those experiencing minimal dilution exhibit homogeneous-like characteristics regardless of altitude. This distinction helps resolve ambiguities in interpreting in situ observations where mixing history is often unknown. Finally, we propose a combined analytical–empirical formulation that captures the relative dispersion during both growth and evaporation.

Atmospheric chemistry and physicsVol. 26(8)
Cooperative Institute for Research in Environmental Sciences (US), University of Colorado Boulder (US), NOAA Chemical Sciences Laboratory (US), Freie Universität Berlin (DE), Ludwig-Maximilians-Universität München (DE)
Deutsche Forschungsgemeinschaft
Life below water
Openalex Percentile: Top 13%
Atmospheric aerosols and clouds
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