Aging of droplet size distribution in stratocumulus clouds: regimes of droplet size distribution evolution
Abstract. The climatic impact of maritime stratocumulus clouds depends on the evolution of their droplet size distribution (DSD), yet the mechanisms controlling their variability during evaporation remain poorly constrained. Using large-eddy simulations coupled with a Lagrangian cloud model, we demonstrate that the DSD evolution follows two primary regimes: adiabatic growth and entrainment–descent. Within the latter, DSD evolution follows divergent pathways determined by the parcel's entrainment history: strong entrainment-driven dilution near the cloud top causes rapid broadening, whereas large-scale boundary-layer descent leads to gradual evaporation. Our Lagrangian analysis of the Damköhler number reveals that the commonly observed vertical transition from inhomogeneous to homogeneous mixing signatures does not necessarily reflect a change in the local mixing mechanism. Instead, it results from the vertical sorting of parcels with divergent histories. Parcels subject to strong entrainment retain inhomogeneous signatures throughout their descent, while those experiencing minimal dilution exhibit homogeneous-like characteristics regardless of altitude. This distinction helps resolve ambiguities in interpreting in situ observations where mixing history is often unknown. Finally, we propose a combined analytical–empirical formulation that captures the relative dispersion during both growth and evaporation.
Authors
- Fabian Hoffmann (ORCID: https://orcid.org/0000-0001-5136-0653)
- Jung-Sub Lim
Institutions
- Cooperative Institute for Research in Environmental Sciences (US)
- University of Colorado Boulder (US)
- NOAA Chemical Sciences Laboratory (US)
- Freie Universität Berlin (DE)
- Ludwig-Maximilians-Universität München (DE)
Publication Details
- Journal
- Atmospheric chemistry and physics
- Published
- 2026-04-22
- DOI
- https://doi.org/10.5194/acp-26-5427-2026
- Primary Topic
- Atmospheric aerosols and clouds
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Deutsche Forschungsgemeinschaft