In Situ Photopolymerization of Hydrogels in Radical Covalent Organic Frameworks
, and fully recoverable large deformation (up to 1500% strain). This exceptional performance is attributed to the physical nanoconfined effect of the framework and chemical crosslinking between hydrogels and COF walls. Furthermore, the exceptional strength, toughness, and durability of the hydrogel enable its excellent applicability in wearable sensors, delivering multiangle detection with high sensitivity over prolonged operation.
Authors
- Wei Zhai (ORCID: https://orcid.org/0000-0003-2307-5243)
- Kun Wu (ORCID: https://orcid.org/0000-0002-2357-3288)
- Chunqing Ji (ORCID: https://orcid.org/0000-0002-5944-3450)
- Wei Juan Zhao (ORCID: https://orcid.org/0000-0003-0265-2590)
- Mounib Bahri (ORCID: https://orcid.org/0000-0002-8336-9158)
- Haobo Qi (ORCID: https://orcid.org/0009-0000-4377-3589)
- Shiqiang Cheng
- Zekun Wang (ORCID: https://orcid.org/0000-0003-3792-535X)
- Nigel D. Browning (ORCID: https://orcid.org/0000-0003-0491-251X)
- Weiwei Zhang (ORCID: https://orcid.org/0000-0002-0378-9946)
- Xiansong Shi (ORCID: https://orcid.org/0000-0002-4258-7941)
- Jing Yang (ORCID: https://orcid.org/0000-0002-3731-368X)
- Peiyao Yan (ORCID: https://orcid.org/0000-0001-7377-1808)
- Zhenkun Li
- Dan Zhao (ORCID: https://orcid.org/0000-0002-4427-2150)
- Binting Huang
- Chaobin He (ORCID: https://orcid.org/0000-0001-8200-8337)
- Qiang Zhu
- Xinyu Dong
Institutions
- East China University of Science and Technology (CN)
- University of Liverpool (GB)
- National University of Singapore (SG)
- Université Bourgogne Franche-Comté (FR)
- Materials Design (France) (FR)
- Advanced Energy Materials (United States) (US)
Publication Details
- Journal
- Journal of the American Chemical Society
- Published
- 2026-04-22
- DOI
- https://doi.org/10.1021/jacs.5c21333
- Primary Topic
- Covalent Organic Framework Applications
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Agency for Science, Technology and Research
- National Research Foundation Singapore
- DSO National Laboratories - Singapore
- Ministry of Education - Singapore
- Public Utilities Board - Singapore
- Science and Technology Support Program of Jiangsu Province