Ultrastrong Light–Matter Coupling in Near-Field Coupled Split-Ring Resonators Revealed by Photocurrent Spectroscopy

Landau polaritons arising from the coupling between cyclotron resonance and terahertz split-ring resonators (SRRs) have served as a central platform for exploring ultrastrong light–matter interaction for more than a decade. Over this period, a wide variety of SRR architectures, differing in size, geometry, and even material composition, have been investigated. However, the regime of near-field coupled SRRs has remained largely unexplored. Here, we demonstrate ultrastrong coupling using photocurrent spectroscopy in two prototypical near-field configurations: an SRR dimer and a topological SRR chain. The measurements reveal hybridization not only with bright resonant modes but also with optically dark modes and topological edge modes, highlighting the exceptional sensitivity and spatial selectivity of the photocurrent spectroscopy. Such engineered near-field interactions allow the study of multimode ultrastrong coupling and the interplay between topological band structure and cavity quantum electrodynamics.